Demineralizing Biomass for Ionic Liquid Cellulose Dissolution

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Solution Overview

Problem

Existing processes struggle to dissolve cellulose from biomass materials containing minerals in Ionic Liquid media due to mineral interference with solvent properties, which affects the efficiency and viability of cellulose regeneration, derivatization, or conversion.

Innovation Solution

A process involving demineralization of biomass materials before contacting them with an Ionic Liquid medium, using a solvent and mechanical action to remove minerals, followed by using inorganic molten salt hydrates as the preferred Ionic Liquid medium, which are more temperature stable and effective in dissolving cellulose even in the presence of water.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If lower grade biomass materials containing minerals are used as feedstock, then cost is reduced and availability is improved, but the minerals interact with the Ionic Liquid medium and change its solvent properties, reducing dissolution efficiency

Engineering Contradiction:
Improvefeedstock availabilityVSAvoidsolvent property stability
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent applies preliminary demineralization treatment to the biomass material before dissolving it in the Ionic Liquid medium. This pre-treatment removes minerals that would otherwise interact with and alter the solvent properties of the Ionic Liquid, ensuring stable dissolution conditions while allowing the use of lower grade, more abundant biomass feedstocks

Inventive Principle:
Principle #10Preliminary action

2Reliability

If demineralization treatment is applied to remove minerals from biomass material, then solvent property stability is improved, but additional process steps are required, increasing process complexity

Engineering Contradiction:
Improvesolvent property stabilityVSAvoidprocess complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent employs aqueous acid solutions that serve multiple functions: they act as demineralization agents to remove minerals, and the water contained in these acid solutions simultaneously serves as an anti-solvent for cellulose precipitation. This multi-functionality reduces the need for additional separate process steps and materials

Inventive Principle:
Principle #6Universality (Multi-functionality)

3Adaptability or versatility

If aqueous acid solutions are used for demineralization, then mineral removal is achieved and water acts as anti-solvent for cellulose, but acid handling requirements increase safety concerns

Engineering Contradiction:
Improvedemineralization effectivenessVSAvoidsafety hazards
Core Design Contradiction:
Adaptability or versatilityVSObject-affected harmful factors

Solution Approach 1:

The patent utilizes the dual role of water in the aqueous acid solution: as a vehicle for acid delivery during demineralization, and subsequently as an anti-solvent for cellulose precipitation. By leveraging this parameter change and multi-functionality, the process achieves effective mineral removal while utilizing readily available materials, though acid handling safety remains a consideration

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process effectively dissolves cellulose from biomass materials while maintaining solvent stability, allowing for efficient regeneration, derivatization, or conversion of cellulose, and enables recycling of the Ionic Liquid medium, enhancing the feasibility of cellulose processing.

Implementation Method 1

contacting the at least partially demineralized biomass material from step (ii) with an Ionic Liquid medium, thereby dissolving at least part of the cellulose component of the biomass material

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentUS8652261B2Process for dissolving cellulose-containing biomass material in an ionic liquid medium
Publication Date: 2014.02.18 MARD INC

AI summary

A process is disclosed for dissolving the cellulose component if a cellulose-containing biomass material in an Ionic Liquid medium. The biomass material contains minerals. At least part of the minerals are removed prior to contacting the biomass material with the Ionic Liquid medium. The Ionic Liquid medium preferably is an inorganic molten salt hydrate.