Biopolymer Acrylic Copolymer Blends for Melt Processing

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Solution Overview

Problem

Biopolymers, such as polylactide, exhibit poor metal release when heated above their glass transition or melting temperatures, leading to difficulties in melt processing techniques like injection molding and calendering due to metal sticking issues, and existing acrylic copolymer processing aids have not significantly improved melt strength in polymers like polycarbonate.

Innovation Solution

A biopolymer composition comprising 85-99.9% biopolymers and 0.1-15% acrylic copolymers, specifically designed to enhance metal release and melt strength, where the acrylic copolymers include a blend of acrylic and methacrylic monomers with varying molecular weights, are used as process aids to improve processing properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If biopolymers are heated above glass transition or melting temperature for melt processing, then processing capability is improved, but metal release deteriorates due to poor sticking release

Engineering Contradiction:
Improvemelt processing capabilityVSAvoidmetal sticking
Core Design Contradiction:
Ease of manufactureVSObject-generated harmful factors

Solution Approach 1:

An acrylic copolymer processing aid is introduced as an intermediary substance between the biopolymer and metal processing equipment. This processing aid modifies the interface interactions, enabling the biopolymer to be processed at temperatures above its glass transition or melting temperature without adhering to metal surfaces, thus resolving the metal sticking problem while maintaining melt processing capability

Inventive Principle:
Principle #24Intermediary (Mediator)

2Object-generated harmful factors

If acrylic copolymer processing aids are added to improve metal release, then metal release is improved, but melt strength does not significantly improve

Engineering Contradiction:
Improvemetal releaseVSAvoidmelt strength
Core Design Contradiction:
Object-generated harmful factorsVSStrength

Solution Approach 1:

The patent optimizes specific parameters of the acrylic copolymer processing aid, including its molecular weight (20,000-500,000 g/mol), composition (acrylic and/or methacrylic monomers with 0-80% styrene), and concentration (0.1-5% by weight). These parameter changes enable the processing aid to simultaneously improve metal release and enhance melt strength, unlike conventional processing aids that only address metal release

Inventive Principle:
Principle #35Parameter changes

3Productivity

If neat polylactide resin is processed in calendering equipment, then processing is attempted, but metal sticking occurs making processing impossible

Engineering Contradiction:
Improveprocessing feasibilityVSAvoidmetal sticking
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The acrylic copolymer processing aid serves as a mediator that prevents direct contact and adhesion between the polylactide resin and metal calendering equipment. By incorporating this processing aid, the resin can be successfully processed through calendering equipment without the metal sticking that makes neat polylactide processing impossible

Inventive Principle:
Principle #24Intermediary (Mediator)

Data Source

PatentEP1976905B1Blends of biopolymers with acrylic copolymers
Publication Date: 2020.10.14 ARKEMA INC

AI summary

The invention relates to a blend of one or more biopolymers with one or more acrylic copolymers, for the purpose of improving the properties of the biopolymer(s). The biopolymer composition comprises 30-99.9 weight percent of biopolymer(s) and 0.1 to 15 weight percent of one or more acrylic copolymers.