Biphasic Furfural Production via Acid Extraction

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Solution Overview

Problem

Current methods for producing furfural and similar organic compounds from biomass face challenges such as high economic and environmental costs due to the need for acid recovery and thermal degradation, which complicates downstream processing and reduces yields.

Innovation Solution

A closed-loop process is implemented that recycles aqueous streams containing acid from hydrolysis steps, using an acid-catalyzed digestion process followed by a biphasic dehydration reaction to produce furfural, allowing for efficient separation and recovery of valuable intermediates and products.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If concentrated mineral acids are used for complete chemical hydrolysis, then sugar yields are improved, but acid recovery becomes more difficult and expensive

Engineering Contradiction:
Improvesugar yieldVSAvoidacid recovery complexity
Core Design Contradiction:
Quantity of substanceVSDevice complexity

Solution Approach 1:

The patent extracts the acid catalyst from the hydrolysis mixture using an organic solvent (such as toluene or xylene). The acid partitions into the organic phase which is then separated from the aqueous sugar solution, eliminating the need for complex acid recovery systems while maintaining high sugar yields

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

An organic solvent acts as an intermediary carrier to transfer the acid catalyst from the aqueous hydrolysis medium to a separable organic phase. This mediator enables easy acid recovery through phase separation without requiring additional recovery equipment

Inventive Principle:
Principle #24Intermediary (Mediator)

2Ease of operation

If dilute acid processes are used for chemical saccharification, then operational simplicity is improved, but thermal degradation increases and sugar yields decrease

Engineering Contradiction:
Improveprocess simplicityVSAvoidsugar yield
Core Design Contradiction:
Ease of operationVSQuantity of substance

Solution Approach 1:

The patent changes the operational parameters by using dilute acid combined with organic solvent extraction, allowing operation at lower temperatures that prevent thermal degradation while maintaining process simplicity. The acid concentration is optimized to balance ease of operation with prevention of sugar decomposition

Inventive Principle:
Principle #35Parameter changes

3Productivity

If high temperature is used in dilute acid processes, then reaction rate is improved, but thermal degradation of monosaccharides increases and sugar yields decrease

Engineering Contradiction:
Improvereaction rateVSAvoidsugar yield
Core Design Contradiction:
ProductivityVSQuantity of substance

Solution Approach 1:

The patent implements continuous acid extraction into the organic phase during the hydrolysis process, maintaining a low acid concentration in the aqueous phase that prevents thermal degradation while sustaining the reaction rate through continuous catalyst availability

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enhances furfural yields, reduces waste, and lowers operational costs by optimizing reaction conditions and minimizing the loss of valuable compounds, making the process more economically attractive.

Implementation Method 1

subjecting the pentosan-containing biomass material to an acid catalyzed digestion process

Methodology Applied
Scientific EffectAcid-catalyzed hydrolysis: Hydrolysis

Implementation Method 2

separating the dehydration product stream into an aqueous recycle stream and an organic product stream

Methodology Applied
Scientific EffectLiquid-liquid extraction: Liquid-Liquid Extraction

Data Source

PatentEP3180323B1Closed-loop production of furfural from biomass
Publication Date: 2020.07.22 SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ BV
  • EP3180323B1 patent drawingFigure 1
  • EP3180323B1 patent drawingFigure 2
  • EP3180323B1 patent drawingFigure 3

AI summary

Methods and processes for the production of valuable organic products and alcohols from biomass material using a closed-loop process having numerous advantages over prior production methods are described. In the process, the biomass is subjected to acid-catalyzed digestion, followed by a separation of the digestion product stream into a solid product stream and a liquid product stream, the liquid product stream thereafter undergoing acid-catalyzed dehydration in the presence of an organic solvent, and thereafter separating the organic products in the organic layer from the aqueous layer. During the process, aqueous and organic fluid streams are fed back into various portions of the production process to increase the concentration of active portions and maximize product recovery.