N,N-Bis[2-hydroxidebenzyl]amine Catalysts for Olefin Polymerization

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Solution Overview

Problem

Current catalyst systems for olefin polymerization, such as chromium-based, metallocene-based, and Ziegler-Natta systems, face limitations in producing high-quality polyolefins with specific properties, particularly in terms of molecular weight distribution and polymerization efficiency.

Innovation Solution

Development of catalyst compositions employing amine bis(phenolate) or N,N-bis[2-hydroxidebenzyl]amine transition metal compounds, which are used in combination with activator-supports and co-catalysts like organoaluminum compounds to enhance olefin polymerization processes, resulting in improved polymer properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional catalyst systems (chromium-based, metallocene-based, Ziegler-Natta) are used for olefin polymerization, then commercial viability is achieved, but molecular weight distribution control and polymerization efficiency are limited

Engineering Contradiction:
Improvepolymerization efficiencyVSAvoidmolecular weight distribution control
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent employs transition metal compounds with specific ligand structures (amines, bis(phenolates), beta-diketonates) that fundamentally change the chemical parameters of the catalyst system. These ligand modifications enable precise control over polymerization kinetics and active site characteristics, achieving both high productivity and narrow molecular weight distributions that conventional catalysts cannot simultaneously provide

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The catalyst system combines transition metal compounds with organic ligands (amines, phenolates, beta-diketonates) to create composite catalyst structures. This composite approach integrates the high activity of transition metals with the structural control capabilities of organic ligands, resulting in catalysts that simultaneously achieve high polymerization efficiency and precise molecular weight distribution control

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of these catalyst compositions leads to the production of polyolefins with controlled molecular weight distributions and enhanced polymerization efficiency, enabling the creation of high-quality homopolymers and copolymers suitable for various applications.

Implementation Method 1

Catalyst compositions containing N,N-Bis[2-hydroxidebenzyl]amine transition metal compounds for the polymerization of olefins

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP2797934B1Catalyst compositions containing n,n-BIS[2-hydroxidebenzyl]amine transition metal compounds for the polymerization of olefins
Publication Date: 2016.08.03 CHEVRON PHILLIPS CHEMICAL COMPANY LP
  • EP2797934B1 patent drawingFigure 1
  • EP2797934B1 patent drawingFigure 2
  • EP2797934B1 patent drawingFigure 3

AI summary

Catalyst compositions containing N,N-bis[2-hydroxidebenzyl]amine transition metal compounds are disclosed. Methods for making these transition metal compounds and for using such compounds in catalyst compositions for the polymerization of olefins also are provided. wherein: M is Ti, Zr, or Hf; X 1 and X2 independently are a monoanionic ligand; each RB and RC independently is a halide, a C1 to C36 hydrocarbyl group, a C1 to C36 halogenated hydrocarbyl group, a C1 to C36 hydrocarboxy group, or a C1 to C36 hydrocarbylsilyl group, wherein p and q independently are 0, 1, 2, 3, or 4; and R A is a C1 to C36 hydrocarbyl group or C1 to C36 halogenated hydrocarbyl group.