Block Copolymer Vertical Alignment

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Solution Overview

Problem

Existing block copolymers face challenges in achieving vertical alignment on various surfaces without pre-treatment, and their phase separation efficiency is limited by conventional methods, particularly on hydrophobic and hydrophilic surfaces.

Innovation Solution

The development of a block copolymer with specific molecular weight and composition parameters that allow for vertical alignment on both hydrophobic and hydrophilic surfaces through thermal annealing, exhibiting in-plane phase diffraction patterns in GISAXS analysis, enhancing self-assembling and phase separation properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If conventional block copolymers are used without pre-treatment, then the manufacturing process is simple, but vertical alignment on diverse surfaces cannot be achieved

Engineering Contradiction:
Improvesimplicity of manufacturing processVSAvoidvertical alignment on diverse surfaces
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent modifies the chemical composition parameters of the block copolymer by incorporating fluorinated groups with specific electronegativity values and arranging hydrophobic and hydrophilic blocks in alternating sequences. This parameter change enables the material to achieve vertical alignment on diverse surfaces without pre-treatment, resolving the contradiction between manufacturing simplicity and alignment precision.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite block copolymer structure combining fluorinated blocks, hydrophobic blocks, and hydrophilic blocks in a multi-block architecture. This composite material design provides both hydrophobic and hydrophilic domains that can interact with diverse surfaces, enabling vertical alignment while maintaining process simplicity.

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If block copolymers are designed for vertical alignment, then alignment performance improves, but the complexity of polymer synthesis increases

Engineering Contradiction:
Improvevertical alignment performanceVSAvoidcomplexity of polymer synthesis
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent divides the polymer into distinct functional segments: fluorinated blocks for surface interaction, hydrophobic blocks for water-repellent domains, and hydrophilic blocks for water-attracting domains. This segmentation allows each block to perform its specific function independently, achieving vertical alignment while using well-established polymerization techniques for each segment.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent optimizes specific parameters including the number of repeating units in each block (5-50), the molecular weight ratios between blocks (1:4 to 4:1), and the electronegativity of fluorinated groups (0.4-0.6). These controlled parameter changes achieve vertical alignment without requiring overly complex synthesis procedures.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If phase separation is enhanced for nanostructure formation, then self-assembling properties improve, but control over domain size and shape becomes more difficult

Engineering Contradiction:
Improveself-assembling and phase separation propertiesVSAvoidcontrol over domain size and shape
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent precisely controls phase separation and domain morphology by adjusting parameters including the molecular weight of each block (affecting domain size), the volume fraction of hydrophobic versus hydrophilic blocks (affecting domain shape), and the degree of fluorination (affecting phase separation efficiency). This parameter optimization enables reliable self-assembly with controlled nanostructure dimensions.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The multi-block composite structure with alternating hydrophobic and hydrophilic segments provides built-in templates for phase separation. The fluorinated blocks enhance the contrast in interfacial energy, promoting sharp phase separation while the controlled block lengths and ratios ensure domain sizes and shapes remain within desired ranges.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The block copolymer demonstrates improved self-assembling and phase separation properties, achieving vertical alignment on diverse surfaces without pre-treatment, and shows enhanced phase separation efficiency with thermal annealing, forming nano-scaled structures like spheres, cylinders, and lamellae.

Implementation Method 1

Block copolymers are capable of forming periodically aligned structure such as the sphere, the cylinder or the lamella through phase separations

Methodology Applied
Scientific EffectPhase separation:

Implementation Method 2

the block copolymer can form a nano-scaled structure by a microphase separation

Methodology Applied
Scientific EffectSelf-assembly: Self-Assembly

Implementation Method 3

since lots of substrates are polar and the air is non-polar, a block having more polarity than the other block in the block copolymer wets on the substrate and a block having less polarity than the other block in the block copolymer wets with respect to the interface between the air

Methodology Applied
Scientific EffectWetting: Wetting

Implementation Method 4

the vertical alignment may be accomplished with respect to a large area in a short time by a thermal annealing

Methodology Applied
Scientific EffectThermal annealing: Annealing

Data Source

PatentEP3078689B1Block copolymer
Publication Date: 2020.12.02 LG CHEM LTD
  • EP3078689B1 patent drawingFigure 1
  • EP3078689B1 patent drawingFigure 2
  • EP3078689B1 patent drawingFigure 3~4

AI summary

The present application provides the block copolymers and their application. The present application may provide the block copolymers that have excellent self assembling and phase separation properties and therefore that can be effectively used in various applications. The present application may also provide applications of the block copolymers.