Borosilicate Glass Syringe Cone Coating Adhesion

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Solution Overview

Problem

Conventional cone coatings for borosilicate glass syringes face challenges with adhesion, thermal expansion mismatch, chemical resistance, and lead content limitations, leading to issues like cracking, flaking, and inadequate sealing, which are exacerbated by stricter regulatory requirements for pharmaceutical packaging.

Innovation Solution

A cone coating for borosilicate glass syringes comprising a low-melting glass matrix with a powdered roughness additive, baked below 700°C, achieving a defined surface roughness and thermal expansion matching the glass substrate, while being free from toxic elements like lead, ensuring secure adhesion and tightness without compromising chemical resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If lead-containing glass frit is used to lower baking temperature and improve adhesion, then the coating adheres well to borosilicate glass, but the coating becomes toxic and fails regulatory requirements

Engineering Contradiction:
ImproveadhesionVSAvoidtoxicity
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters of the glass frit, specifically replacing lead oxide with alternative oxides like bismuth oxide, zinc oxide, and boron oxide. This compositional parameter change allows the coating to be baked at lower temperatures (below 700°C) without lead, maintaining adhesion while eliminating toxicity to meet regulatory requirements for pharmaceutical packaging.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite glass frit formulations combining multiple oxide components (bismuth oxide, zinc oxide, boron oxide, silica) to achieve the desired properties. This composite approach allows the coating to exhibit both low melting temperature for good adhesion and lead-free composition for safety, resolving the contradiction between performance and toxicity.

Inventive Principle:
Principle #40Composite materials

2Object-affected harmful factors

If lead-free glass frit is used to eliminate toxicity, then the coating becomes safe for pharmaceutical use, but the thermal expansion mismatch causes cracking and flaking

Engineering Contradiction:
ImprovetoxicityVSAvoidcoating integrity
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

The patent carefully adjusts the chemical composition parameters of the lead-free glass frit to match the thermal expansion coefficient of borosilicate glass. By optimizing the ratios of bismuth oxide, zinc oxide, boron oxide, and silica, the coating's thermal expansion is tuned to be compatible with the substrate, preventing stress-induced cracking and flaking while maintaining lead-free safety.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides a borosilicate glass syringe with enhanced adhesion and sealing capabilities, meeting regulatory standards for pharmaceutical packaging by maintaining chemical resistance and preventing cracking or flaking, while ensuring the coating is environmentally friendly and safe for medical applications.

Implementation Method 1

The glass frit melts and flows during baking

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 2

ensure the adhesion of the baked layer to the glass substrate through diffusion processes

Methodology Applied
Scientific EffectDiffusion: Diffusion

Implementation Method 3

liquid organic components that evaporate or decompose during baking

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 4

liquid organic components that evaporate or decompose during baking

Methodology Applied
Scientific EffectDecomposition: Decomposition (biological)

Data Source

PatentEP2606928B1Borosilicate glass syringe with a cone coating which increases the surface roughness
Publication Date: 2021.03.03 SCHOTT AG
  • EP2606928B1 patent drawingFigure 1
  • EP2606928B1 patent drawing

AI summary

The syringe (1) has a cylinder (2) for accommodating liquid medicament, and a cone (3) comprising borosilicate glass having thermal expansion in the range of about 20 to 300 degrees centigrade of less than 6x 10 ->6/Kelvin. The cone encloses an outlet channel (4) and has an outside surface with a coating (5) exhibiting an increased roughness compared to the outside surface. The coating comprises a glass matrix with structure-forming particles embedded in the matrix, where the glass matrix is free of lead, cadmium, mercury and chromium VI. The coating has roughness of about 0.3 and 2 micrometer.