Bridged Metallocene Catalyst for Ethylene Interpolymer Production Rate

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Solution Overview

Problem

Current solution polymerization processes for producing ethylene interpolymers face challenges in achieving higher production rates, increasing molecular weight at higher reactor temperatures, and efficiently incorporating α-olefins to reduce density and optimize reactor feed ratios.

Innovation Solution

The use of a bridged metallocene catalyst formulation in a continuous solution polymerization process, involving multiple reactors operating at varying temperatures, allows for the production of ethylene interpolymers with improved properties. This formulation includes specific components such as a bulky ligand-metal complex, an alumoxane co-catalyst, a boron ionic activator, and a hindered phenol, optimized in specific molar ratios to enhance catalyst activity and polymer properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Volume of stationary object

If reactor temperature is decreased to increase molecular weight, then polymer molecular weight increases, but solution viscosity becomes too high

Engineering Contradiction:
Improvemolecular weightVSAvoidreactor temperature
Core Design Contradiction:
Volume of stationary objectVSTemperature

Solution Approach 1:

The patent employs a bridged metallocene catalyst formulation that fundamentally changes the kinetic parameters of polymerization, enabling high molecular weight production at elevated temperatures where conventional catalysts would produce low molecular weight polymer due to excessive chain transfer reactions. The catalyst's unique structure maintains high activity and selectivity across a broader temperature range.

Inventive Principle:
Principle #35Parameter changes

2Productivity

If conventional catalyst formulations are used, then production rate is limited, but increasing production rate reduces profitability

Engineering Contradiction:
Improveproduction rateVSAvoidprofitability
Core Design Contradiction:
ProductivityVSLoss of energy

Solution Approach 1:

The bridged metallocene catalyst formulation dramatically increases polymerization rate constants, enabling production rates exceeding 10,000 pounds per hour while maintaining high catalyst efficiency and reducing operating costs through lower catalyst loadings and improved process intensity.

Inventive Principle:
Principle #35Parameter changes

3Quantity of substance

If conventional catalysts are used, then α-olefin incorporation efficiency is low, but increasing α-olefin feed ratio increases process complexity

Engineering Contradiction:
Improveα-olefin incorporationVSAvoidprocess complexity
Core Design Contradiction:
Quantity of substanceVSDevice complexity

Solution Approach 1:

The bridged metallocene catalyst exhibits enhanced comonomer incorporation kinetics, achieving superior α-olefin incorporation efficiency at lower feed ratios. The catalyst's steric and electronic properties favor α-olefin insertion into the growing polymer chain, reducing the need for complex feedstock blending while maintaining desired polymer density and morphology.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in ethylene interpolymer products with increased molecular weight, improved density control, and enhanced production rates, while also reducing the amount of α-olefin required in the reactor feed, thus optimizing process efficiency and product properties.

Implementation Method 1

employing at least one bridged metallocene catalyst formulation to form an ethylene interpolymer product

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP3707170B1Manufacturing ethylene interpolymer products at higher production rate
Publication Date: 2025.05.14 NOVA CHEM (INT) SA
  • EP3707170B1 patent drawingFigure 1
  • EP3707170B1 patent drawingFigure 2
  • EP3707170B1 patent drawingFigure 3

AI summary

This disclosure relates to an improved continuous solution polymerization process wherein production rate is increased. Process solvent, ethylene, optional comonomers, optional hydrogen and a bridged metallocene catalyst formulation are injected into a first reactor to form a first ethylene interpolymer. Optionally, process solvent, ethylene, optional comonomers, optional hydrogen and a bridged metallocene catalyst formulation are injected into a second reactor forming a second ethylene interpolymer. The first and second reactors may be configured in series or parallel modes of operation. Optionally, a third ethylene interpolymer is formed in a third reactor, wherein a homogeneous catalyst formulation or a heterogeneous catalyst formulation is employed. In solution, the first, optional second and optional third ethylene interpolymers are combined, the catalyst is deactivated, the solution is optionally passivated and following a phase separation process an ethylene interpolymer product is recovered.