Bulk Metal Hydrotreating Catalyst for Low Sulfur Distillates

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Solution Overview

Problem

There is a continuous need for improved hydrotreating catalysts and processes to reduce sulfur and nitrogen content in distillate boiling range hydrocarbon streams, as existing technologies struggle to meet increasingly stringent environmental regulations, particularly with the decreasing supply of low sulfur, low nitrogen crudes.

Innovation Solution

A process using a bulk metal hydrotreating catalyst comprising a Group VIB metal component (molybdenum or tungsten), a Group V metal component (vanadium or niobium), and a Group VIII metal component (nickel or cobalt), with a specific molar ratio, to contact distillate boiling range feedstreams with hydrogen-containing gas under effective hydrotreating conditions, effectively removing nitrogen and organically bound sulfur contaminants and hydrogenating aromatics.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional hydrotreating catalysts are used to reduce sulfur and nitrogen content, then environmental regulations are met, but catalyst activity decreases and process conditions become more severe

Engineering Contradiction:
Improvecatalyst activityVSAvoidprocess conditions
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The patent applies composite materials by combining Group VIB metals (molybdenum, tungsten) with Group V metals (vanadium, niobium, tantalum) and Group VIII metals (nickel, cobalt, iron) to create a synergistic catalyst system. This composite approach allows the catalyst to maintain high activity for sulfur and nitrogen removal while operating under milder conditions, resolving the contradiction between catalyst reliability and process severity.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent utilizes parameter changes by optimizing the molar ratio of metal components in the catalyst formulation. By adjusting the ratios of Group VIB, Group V, and Group VIII metals, the catalyst achieves enhanced performance at lower temperatures and pressures, thereby maintaining reliability while reducing process severity.

Inventive Principle:
Principle #35Parameter changes

2Temperature

If more active catalysts are used to meet sulfur and nitrogen limits, then milder process conditions are achieved, but catalyst composition becomes more complex

Engineering Contradiction:
Improveprocess conditionsVSAvoidcatalyst composition
Core Design Contradiction:
TemperatureVSDevice complexity

Solution Approach 1:

The patent applies parameter changes by establishing specific molar ratio ranges for the metal components (Group VIB:Group V:Group VIII = 0.35-2:1) to optimize catalyst performance. This systematic parameter optimization achieves milder operating conditions while maintaining a manageable catalyst composition structure, avoiding excessive complexity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies universality by designing a catalyst system where multiple metal groups perform complementary functions: Group VIB metals provide primary hydrotreating activity, Group V metals enhance stability and selectivity, and Group VIII metals promote nitrogen removal. This multi-functional design achieves mild conditions without requiring overly complex single-component catalysts.

Inventive Principle:
Principle #6Universality (Multi-functionality)

3Duration of action of stationary object

If existing catalyst formulations are used, then sulfur and nitrogen removal is achieved, but catalyst lifespan between regenerations is limited

Engineering Contradiction:
Improvecatalyst lifespanVSAvoidcatalyst activity
Core Design Contradiction:
Duration of action of stationary objectVSReliability

Solution Approach 1:

The patent applies composite materials by integrating multiple metal groups with complementary properties that enhance catalyst stability and longevity. The synergistic interaction between Group VIB, Group V, and Group VIII metals creates a more durable catalyst structure that maintains high activity over extended periods, thereby extending lifespan between regenerations while preserving reliability.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent applies continuity of useful action by designing a catalyst formulation that maintains stable activity over time through the synergistic metal combination. The multi-metal system provides continuous effective action for sulfur and nitrogen removal without rapid deactivation, extending the operational lifespan between regenerations while sustaining high reliability.

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves a significant reduction in sulfur, nitrogen, and aromatic content in distillate products, meeting regulatory standards and extending catalyst lifespan, while operating under milder conditions, thus enhancing energy efficiency and catalyst activity.

Implementation Method 1

contacting a distillate boiling range feedstream containing aromatics, nitrogen and organically bound sulfur contaminants in a reaction stage with a bulk metal hydrotreating catalyst in the presence of hydrogen-containing treat gas thereby producing a reaction product

Methodology Applied
Scientific EffectHydrotreating: Hydrogenation

Implementation Method 2

bulk metal hydrotreating catalyst comprises: i) a Group VIB metal component selected from molybdenum, tungsten, and mixtures thereof; ii) a Group V metal component selected from vanadium, niobium, tantalum, and mixtures thereof; and iii) a Group VIII metal component selected from nickel, cobalt, iron, and mixtures thereof

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 3

effective hydrotreating conditions are effective at removing at least a portion of the nitrogen and organically bound sulfur contaminants and hydrogenating at least a portion of the aromatics

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Data Source

PatentUS7780845B2Process to manufacture low sulfur distillates
Publication Date: 2010.08.24 EXXONMOBIL TECHNOLOGY & ENGINEERING CO

AI summary

The instant invention relates to a process to produce low sulfur distillate products through the hydrotreating of distillate boiling range feedstreams in the presence of a bulk metal hydrotreating catalyst.