Calendula Extract via Supercritical CO2 for Triterpene Standardization

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Solution Overview

Problem

Existing methods for extracting Calendula officinalis extracts with organic solvents result in low, non-standardized content of triterpene esters, contamination with unnecessary substances, and potential solvent residues, posing formulation challenges and environmental concerns.

Innovation Solution

A process involving the extraction of Calendula officinalis flowers with carbon dioxide in a supercritical phase at specific conditions (temperature 60-70°C and pressure 600-700 bar) to obtain extracts A and B, which are then mixed in a specific ratio to create a standardized triterpene ester mixture for use in topical formulations.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If extraction with organic solvent is used, then the extraction process is simple, but the extract contains low and non-standardized content of triterpene esters along with unnecessary substances and solvent residues

Engineering Contradiction:
Improveextraction process simplicityVSAvoidtriterpene ester content standardization
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent applies parameter changes by transitioning from conventional organic solvent extraction to supercritical carbon dioxide extraction, changing the physical state and chemical properties of the extraction medium. This parameter change enables selective extraction of triterpene esters while excluding unnecessary substances, achieving standardized content (at least 3% triterpene esters with faradiol esters representing at least 75% of the total) without solvent residues

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent utilizes phase transitions of carbon dioxide between supercritical and gaseous states to control the extraction process. By adjusting pressure and temperature parameters, CO2 transitions to a supercritical state for extraction, then returns to gaseous state for easy separation from the extract, eliminating the need for solvent removal and preventing solvent residues in the final product

Inventive Principle:
Principle #36Phase transitions

2Reliability

If extraction with carbon dioxide in supercritical phase is used, then the active principles are maintained integral, but further purification stages are required to eliminate undesired components

Engineering Contradiction:
Improveactive principles integrityVSAvoidpurification process complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent optimizes extraction parameters (temperature of 40-50°C and pressure of 300-800 bar) to achieve selective extraction that maintains active principles integrity while minimizing undesired components. By carefully controlling these parameters, the process extracts triterpene esters with high selectivity, reducing the need for further purification stages compared to conventional methods

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If higher pressure and extraction modifier are used in supercritical CO2 extraction, then the content of faradiol myristate is improved, but the process complexity and cost increase

Engineering Contradiction:
Improvefaradiol myristate contentVSAvoidextraction process complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent achieves high faradiol myristate content by optimizing pressure parameters (300-800 bar) and temperature (40-50°C) without requiring extraction modifiers. This parameter optimization approach attains standardized triterpene ester content while avoiding the added complexity and cost associated with modifier addition found in other methods

Inventive Principle:
Principle #35Parameter changes

4Ease of manufacture

If conventional extraction methods are used, then the extraction process is straightforward, but considerable amounts of extract must be used for preparation of finished products

Engineering Contradiction:
Improveextraction process simplicityVSAvoidextract efficiency
Core Design Contradiction:
Ease of manufactureVSProductivity

Solution Approach 1:

The patent improves extract efficiency by changing the extraction method to supercritical CO2 with optimized parameters, achieving standardized triterpene ester content (at least 3%). This concentration standardization means that smaller, more efficient amounts of extract are required for finished product preparation compared to conventional methods that yield dilute, non-standardized extracts

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies selective extraction by using supercritical CO2 to specifically target and extract triterpene esters from Calendula officinalis while leaving unnecessary substances behind. This selective taking out of desired components concentrates the active principles in the extract, improving the efficiency and reducing the quantity needed for final formulations

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process yields a balanced and enriched triterpene ester extract with at least 3% content, ensuring effective lenitive, protective, and anti-reddening action in topical formulations while minimizing unwanted components and solvent residues, thus enhancing product tolerability and stability.

Implementation Method 1

extraction with carbon dioxide in supercritical phase at specific conditions (temperature 60-70°C and pressure 600-700 bar)

Methodology Applied
Scientific EffectSupercritical fluid extraction: Supercritical Fluid Extraction

Implementation Method 2

extraction of Calendula officinalis flowers with carbon dioxide in a supercritical phase

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentEP2520306B1Process for preparing an inflorescence extract of Calendula Officinalis by means of extraction with supercritical carbon dioxide and compositions containing said extract
Publication Date: 2017.12.06 UNIFARCO SPA

AI summary

The present invention regards a process for extracting flowering tops of Calendula officinalis comprising the extraction with carbon dioxide in supercritical phase at high temperature and pressures, in order to obtain two extracts which, when mixed together in suitable weight ratios, constitute a total extract enriched with calenduladiol, arnidiol and faradiol esters with myristic, lauric and/or palmitic acid. This total extract can be conveniently used for preparing topical formulations for cosmetic or pharmaceutical use.