Carbohydrate Etherification via Superheated Steam

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Solution Overview

Problem

Conventional carbohydrate etherification processes require large volumes of solvent, result in high environmental burden due to excessive use of etherification agents and salt, and are limited by low degree of substitution (DS) and restricted molecule identity, making them economically and environmentally inefficient.

Innovation Solution

The process involves subjecting carbohydrates to superheated steam under alkaline conditions in the presence of an etherification agent, eliminating the need for solvents and reducing salt usage, while allowing for higher DS and introduction of novel ether groups, thereby enabling the production of carbohydrate ethers with enhanced properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Adaptability or versatility

If conventional etherification is carried out in polar solvent environment, then the reaction can proceed with various functionalizing molecules, but the solvent volume required is large and the environmental burden increases

Engineering Contradiction:
Improveidentity of etherification moleculeVSAvoidsolvent volume
Core Design Contradiction:
Adaptability or versatilityVSQuantity of substance

Solution Approach 1:

The invention extracts and eliminates the polar solvent from the conventional etherification system, performing the reaction in a solvent-free environment. This resolves the contradiction by removing the harmful substance (solvent) while maintaining the reaction's ability to proceed with various etherification agents through alternative reaction conditions (superheated steam, alkaline catalyst).

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the physical and chemical parameters of the reaction system by using superheated steam instead of polar solvents, and employing alkaline conditions with controlled water content (5-40 wt%). This parameter transformation allows the reaction to proceed without large volumes of solvent while maintaining versatility in etherification agent selection.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If large quantities of etherification agent are used to achieve high DS, then the degree of substitution increases, but the cost increases and large amounts of salt byproduct are produced

Engineering Contradiction:
Improvedegree of substitutionVSAvoidetherification agent quantity
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The invention introduces an alkaline catalyst as an intermediary that facilitates the etherification reaction, enabling higher degree of substitution with reduced etherification agent consumption. The catalyst activates the reaction pathway, allowing more efficient utilization of the etherification agent and reducing waste.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

By changing the reaction parameters to include alkaline conditions and controlled water content, the invention achieves higher DS with lower etherification agent quantities. The modified reaction environment improves the efficiency and selectivity of the etherification process.

Inventive Principle:
Principle #35Parameter changes

3Stability of the object's composition

If salt is added during reaction to retain starch granular structure, then the structure is preserved, but the environmental burden increases

Engineering Contradiction:
Improvestarch granular structureVSAvoidenvironmental burden
Core Design Contradiction:
Stability of the object's compositionVSObject-generated harmful factors

Solution Approach 1:

The invention extracts and eliminates the need for salt addition by performing etherification under alkaline conditions with controlled water content. This removes the harmful substance (salt) from the process while maintaining starch granular structure through alternative stabilization mechanisms.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The starch granular structure stabilizes itself under the alkaline reaction conditions with controlled water content, without requiring external salt addition. The system self-regulates to maintain structural integrity during the etherification process.

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method achieves higher DS with reduced environmental impact, preserves starch granular structure, and enables the creation of carbohydrate ethers that could not be previously synthesized, offering economic and environmental benefits along with expanded molecular diversity.

Implementation Method 1

subjecting the carbohydrate to superheated steam under alkaline conditions in the presence of an etherification agent

Methodology Applied
Scientific EffectSuperheated steam: Superheating

Data Source

PatentEP3405472B1Etherification of carbohydrates using superheated steam
Publication Date: 2020.01.01 STICHTING WAGENINGEN RES

AI summary

The invention pertains to a method for the etherification of a carbohydrate, comprising subjecting the carbohydrate to superheated steam under alkaline conditions in the presence of an etherification agent to obtain a carbohydrate ether.