Carbon Negative Electrode Material for Lithium Secondary Battery

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Solution Overview

Problem

Lithium secondary batteries face issues with battery short circuits and explosion risks due to dendrite formation, and the use of carbon-based active materials leads to particle deformation during the rolling process, deteriorating the battery's lifespan characteristics.

Innovation Solution

A carbon-based negative electrode active material is developed, satisfying specific density and sphericity criteria to minimize particle deformation during the rolling process, using natural or artificial graphite with a Raman R value of 0.01 to 1.4, and including hard or soft carbon in 5-15 wt%, which reduces resistance and improves capacity retention.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If carbon-based active material is used for negative electrode, then battery safety is improved (no dendrite formation), but particle deformation occurs during rolling process leading to deteriorated lifespan characteristics

Engineering Contradiction:
Improvebattery safetyVSAvoidlifespan characteristics
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The invention changes the physical parameters of the carbon-based active material particles, specifically controlling sphericity (0.7-1.0), pellet density (1.0-1.5 g/cm³), and tap density (0.8-1.2 g/cm³) to satisfy a specific relational expression. These parameter adjustments minimize particle deformation during the rolling process while maintaining battery safety, thereby improving lifespan characteristics without sacrificing reliability.

Inventive Principle:
Principle #35Parameter changes

2Duration of action of stationary object

If particle deformation is minimized during rolling, then lifespan characteristics are improved, but manufacturing process complexity increases due to specific density and sphericity requirements

Engineering Contradiction:
Improvelifespan characteristicsVSAvoidmanufacturing process complexity
Core Design Contradiction:
Duration of action of stationary objectVSDevice complexity

Solution Approach 1:

The invention establishes specific parameter ranges for sphericity (0.7-1.0), pellet density (1.0-1.5 g/cm³), and tap density (0.8-1.2 g/cm³) that satisfy a relational expression. By defining these parameters upfront, the manufacturing process becomes more controlled and predictable, reducing variability and actually simplifying quality assurance while achieving minimal particle deformation and improved lifespan characteristics.

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentUS20220238880A1Negative Electrode Active Material for Secondary Battery and Secondary Battery Including the Same
Publication Date: 2022.07.28 SK ON CO LTD

AI summary

Provided is a negative electrode active material for a secondary battery including a carbon-based active material. The negative electrode active material satisfies the following Relational Expression 1, [Relational Expression 1] 0.1≤(Dp−DT)/sphericity≤0.28 where Dp is a pellet density (g/cm3) of the carbon-based active material, DT is a tap density (g/cm3) of the carbon-based active material, and the sphericity is a sphericity of a particle of the carbon-based active material.