cBN Grain Feature Control via HPHT Phase Transition

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Solution Overview

Problem

Current methods for producing cubic boron nitride (cBN) grains from hexagonal boron nitride (hBN) under high pressures and temperatures often result in grains with defects and limited control over unique features, affecting their abrasive properties.

Innovation Solution

A method involving a high-pressure and high-temperature process using a catalyst system, where the reaction mixture includes a source of boron, nitrogen, and a catalyst metal, with controlled pressure and temperature conditions to form cBN grains, followed by chemical and physical separation and cleaning processes to enhance grain features and properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional high-pressure high-temperature methods are used to produce cBN grains, then cBN grains can be formed, but the grains have defects and limited control over unique features

Engineering Contradiction:
Improvecontrol over grain featuresVSAvoidgrain defects
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent applies preliminary action by pre-forming hexagonal boron nitride (hBN) grains with controlled morphology and size before subjecting them to high-pressure high-temperature treatment. This pre-preparation step allows better control over the final cBN grain features, reducing defects and enabling more precise control over grain characteristics compared to starting with raw materials.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent employs parameter changes by systematically varying pressure, temperature, and holding time parameters during the HPHT treatment of hBN grains. By optimizing these parameters (e.g., pressures of 5-15 GPa, temperatures of 1500-2500°C, and specific holding times), the process achieves better control over cBN grain formation, reducing defects and creating unique surface features that improve performance.

Inventive Principle:
Principle #35Parameter changes

2Strength

If conventional cBN grains are used, then abrasive properties are limited, but modifying the production process increases process complexity

Engineering Contradiction:
Improveabrasive performanceVSAvoidprocess complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent applies segmentation by dividing the production process into distinct stages: (1) preparation of hBN precursor grains with controlled morphology, (2) HPHT treatment to convert hBN to cBN, and (3) post-treatment to develop unique surface features. This segmented approach allows optimization of each stage independently, achieving superior abrasive performance while managing overall process complexity through systematic organization.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent utilizes composite materials by combining hBN precursor grains with catalyst systems during the HPHT treatment. The catalyst system (containing metals such as Fe, Ni, Co, or their sulfides/nitrides) works synergistically with the hBN to facilitate the phase transformation and create cBN grains with enhanced properties, effectively creating a composite processing system that improves abrasive performance.

Inventive Principle:
Principle #40Composite materials

3Reliability

If standard recovery methods are used, then cBN grains can be separated, but unique features and retention force are not optimized

Engineering Contradiction:
Improveretention force in bondVSAvoidgrain feature development
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent applies periodic action through controlled heating and cooling cycles during and after the HPHT treatment. The process includes holding at peak pressure and temperature for specific durations, followed by controlled cooling rates. This periodic thermal treatment promotes the development of unique surface features on cBN grains, such as concave indentations and peaks, which enhance retention force in bond materials while maintaining manufacturing precision.

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method produces cBN grains with unique features such as concave indentations, peaks, and valleys, improving their retention force in bond materials and enhancing their performance in grinding applications, demonstrated by improved grinding performance and surface finish compared to conventional cBN grains.

Implementation Method 1

hexagonal boron nitride (hBN) grains are subjected to a high-pressure and high-temperature process using a catalyst system to effect the phase transition

Methodology Applied
Scientific EffectPhase transition: Phase Change

Implementation Method 2

The reaction mass is maintained under pressure and temperature conditions that thermodynamically favor the formation of cubic boron nitride crystals

Methodology Applied
Scientific EffectThermodynamic transformation: Phase Change

Data Source

PatentEP3660121B1Method of making a plurality of cubic boron nitride having unique features
Publication Date: 2024.05.01 DIAMOND INNOVATIONS INC
  • EP3660121B1 patent drawingFigure 1~3
  • EP3660121B1 patent drawingFigure 4
  • EP3660121B1 patent drawingFigure 5

AI summary

An uncoated abrasive or superabrasive grain having at least one grain face including three or more features projecting from the grain face wherein the height (h) and the lateral length (1) of each feature is greater than about 0.1 micron.