Acid Bleaching of Reclaimed Cellulose for Low-Clogging Regeneration

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Solution Overview

Problem

Existing methods for regenerating cellulose are inefficient and costly, with a high propensity for clogging due to metal content, requiring multiple stages and the use of complex agents like EDTA, which poses environmental concerns.

Innovation Solution

A one-stage process combining acid metal removal and acid oxidative bleaching to efficiently reduce metal content and clogging in reclaimed cellulose fibers, eliminating the need for additional bleaching and metal removal steps, using acids like hydrochloric, formic, or acetic acid, and oxidative agents like hydrogen peroxide or ozone.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If multiple stages are used for metal removal and bleaching, then metal content and clogging are reduced, but process complexity and cost increase

Engineering Contradiction:
Improvemetal content and cloggingVSAvoidprocess complexity
Core Design Contradiction:
Object-affected harmful factorsVSDevice complexity

Solution Approach 1:

The patent combines acid metal removal and acid oxidative bleaching into a single integrated stage, where both functions are performed simultaneously using the same acidic environment and oxidative agents, eliminating the need for separate treatment stages while achieving both metal removal and bleaching objectives

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The acidic oxidative treatment stage serves multiple functions simultaneously: it acts as both a metal removal agent through acid dissolution and a bleaching agent through oxidative reactions, making the process step multi-functional and reducing overall process complexity

Inventive Principle:
Principle #6Universality (Multi-functionality)

2Object-affected harmful factors

If EDTA is used for metal removal, then metal content is reduced, but environmental harm increases

Engineering Contradiction:
Improvemetal contentVSAvoidenvironmental harm
Core Design Contradiction:
Object-affected harmful factorsVSObject-generated harmful factors

Solution Approach 1:

The patent replaces the environmentally harmful EDTA chelating agent with environmentally benign acidic oxidative agents that achieve metal removal through acid dissolution and oxidation mechanisms, converting the harmful chemical approach into a more sustainable process that eliminates persistent environmental contaminants

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The patent uses readily available, inexpensive acidic agents (such as sulfuric acid, hydrochloric acid, or organic acids) and oxidative agents (such as hydrogen peroxide, sodium hypochlorite, or ozone) that can be easily degraded in the environment, replacing expensive and persistent EDTA with simpler, more environmentally friendly alternatives

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Object-affected harmful factors

If multiple treatment stages are used, then metal removal efficiency is improved, but processing time increases

Engineering Contradiction:
Improvemetal contentVSAvoidprocessing time
Core Design Contradiction:
Object-affected harmful factorsVSLoss of time

Solution Approach 1:

The patent merges acid metal removal and acid oxidative bleaching into a single simultaneous treatment stage, where both metal dissolution and oxidative bleaching occur concurrently in the same reactor under the same conditions, thereby reducing total processing time while maintaining effective metal removal

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent implements a continuous single-stage process where acid metal removal and oxidative bleaching proceed simultaneously without interruption or intermediate steps, maintaining continuous useful action throughout the treatment period and eliminating time losses associated with stage transitions

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly reduces clogging and metal content in regenerated cellulose, making the process faster, more efficient, and cost-effective, while avoiding the environmental issues associated with EDTA, by oxidizing and removing metal ions in a single stage.

Implementation Method 1

acid metal removal

Methodology Applied
Scientific EffectAcid dissolution:

Implementation Method 2

treatment with a complexing agent

Methodology Applied
Scientific EffectComplexation:

Implementation Method 3

acid oxidative bleaching

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 4

oxidative bleaching stage can be treatment with peroxide, oxygen or ozone

Methodology Applied
Scientific EffectPhoto-oxidation: Photo-oxidation

Implementation Method 5

exposing the cellulose containing material to oxygen with an alkali aqueous solution

Methodology Applied
Scientific EffectHydration:

Implementation Method 6

swelling the cellulose

Methodology Applied
Scientific EffectSwelling:

Implementation Method 7

bleached with ozone at acid conditions

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 8

oxidative agents like hydrogen peroxide or ozone

Methodology Applied
Scientific EffectRedox reactions: Redox Reactions

Implementation Method 9

oxidizing and removing metal ions

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentUS20230146394A1One stage method for acid metal removal and bleach
Publication Date: 2023.05.11 CIRCULOSE AB

AI summary

There is provided a process for chemically pretreating reclaimed cellulose fibres to be used in the production of moulded bodies from regenerated cellulose, wherein the pretreatment includes one stage, in which stage acid metal removal and acid oxidative bleaching are carried out together. Advantages include that the propensity of the regenerated cellulose to clog when flowing in a tube and through a nozzle is reduced. This is believed to be an effect of an efficient metal removal. The need for additional bleaching steps and/or metal removing steps is reduced or even eliminated. A one-stage method is more efficient, faster and less costly compared to a multi-stage method according to the prior art. From an environmental perspective, acidic metal removal is preferred over removal by chelating agents such as EDTA.