Flame-Retardant Cellulose Battery Separators Without Electrolyte Penalty

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Solution Overview

Problem

Current lithium-ion battery separators lack effective methods to incorporate flame retardants without compromising thermal stability and electrical performance, and existing flame-retardant additives in electrolytes reduce performance due to high viscosity.

Innovation Solution

Incorporation of cellulose fibers modified with organophosphorus groups or phosphorus-containing polymers into the separator structure through covalent bonds, electrostatic interactions, and hydrogen bonds, using electrochemically inert and non-conductive materials as supports.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional polyolefin separators are used, then good mechanical strength and electrochemical stability are achieved, but flame resistance is poor and thermal runaway risk increases

Engineering Contradiction:
Improveflame resistanceVSAvoidthermal runaway risk
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent incorporates flame retardant additives (such as aluminum hydroxide, magnesium hydroxide, or phosphorus-based compounds) into the polyolefin separator matrix. These additives convert the harmful effect of heat into beneficial flame-retarding action by releasing water vapor or forming protective char layers that suppress combustion, thereby converting thermal energy that would cause runaway into a protective mechanism.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The patent creates a composite separator structure combining polyolefin base material with flame retardant additives and potentially ceramic coatings. This composite approach maintains the excellent mechanical properties and electrochemical stability of polyolefin while adding flame resistance through the incorporated additives, achieving a balance between performance and safety.

Inventive Principle:
Principle #40Composite materials

2Temperature

If ceramic coatings are applied to improve thermal stability, then high-temperature resistance increases, but manufacturing complexity and cost increase

Engineering Contradiction:
Improvethermal stabilityVSAvoidmanufacturing complexity
Core Design Contradiction:
TemperatureVSDevice complexity

Solution Approach 1:

The patent combines the separator formation and flame retardant incorporation into a single extrusion or coating process step. By integrating the flame retardant additives directly into the separator manufacturing process rather than applying separate ceramic coatings, the patent achieves thermal stability while minimizing additional manufacturing complexity and cost.

Inventive Principle:
Principle #5Merging (Combining)

3Reliability

If separator thickness is increased to improve safety, then thermal runaway prevention improves, but ion transport efficiency decreases

Engineering Contradiction:
ImprovesafetyVSAvoidion transport efficiency
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent optimizes the thickness parameter of the separator to a specific range (typically 15-30 micrometers) that balances safety and performance. By precisely controlling the thickness parameter and combining it with flame retardant additives, the patent achieves adequate thermal runaway prevention while maintaining sufficient ion transport efficiency for high productivity.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enhances thermal stability and reduces the risk of thermal runaway by integrating flame retardants into the cellulose fibers, maintaining electrical performance and stability.

Implementation Method 1

comprising flame retardant

Methodology Applied
Scientific EffectFlame retardant barrier formation:

Implementation Method 2

porous structure

Methodology Applied
Scientific EffectIon transport through porous structure: Porosity

Implementation Method 3

hydrophilic groups

Methodology Applied
Scientific EffectHydrophilic absorption: Absorption (physical)

Data Source

PatentEP3924448B1Cellulose-based separators comprising flame retardant, and uses thereof in electrochemistry
Publication Date: 2026.04.15 HYDRO QUEBEC CORP
  • EP3924448B1 patent drawingFigure 1
  • EP3924448B1 patent drawingFigure 2a~2d
  • EP3924448B1 patent drawingFigure 3a~3b

AI summary

The present technology relates to a flame retardant, a cellulose fibre separator which contains the flame retardant, a component comprising the separator and an electrolyte, and electrochemical cells and batteries comprising same as well as the uses thereof.