Cement Admixture Copolymer Layered Double Hydroxide Corrosion

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Solution Overview

Problem

Conventional cement admixtures, particularly polycarboxylic acid (PCA)-based admixtures, face challenges in maintaining both dispersibility and workability over time, and they lack sufficient corrosion resistance, especially in marine concrete structures where chloride ions can cause corrosion.

Innovation Solution

A cement admixture is developed using a polycarboxylic acid-based copolymer derived from a macromonomer and a layered double hydroxide, which is prepared by reacting a compound with a saturated or unsaturated dicarboxylic acid, an anhydride, or their mixture, under specific conditions to enhance dispersibility and workability while providing corrosion resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Duration of action of stationary object

If the molecular structure of PCA-based admixture is modified to improve workability maintenance, then workability maintenance is improved, but dispersibility is considerably reduced

Engineering Contradiction:
Improveworkability maintenanceVSAvoiddispersibility
Core Design Contradiction:
Duration of action of stationary objectVSManufacturing precision

Solution Approach 1:

The patent combines polycarboxylic acid-based copolymer with layered double hydroxide to create a composite cement admixture. The copolymer provides dispersibility through steric hindrance repulsion from polyethylene oxide side chains, while the layered double hydroxide structure enhances workability maintenance. This composite approach allows both dispersibility and workability maintenance to be improved simultaneously rather than requiring a trade-off between them.

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If dispersibility of PCA-based admixture is improved, then dispersibility is improved, but workability maintenance is considerably reduced

Engineering Contradiction:
ImprovedispersibilityVSAvoidworkability maintenance
Core Design Contradiction:
Manufacturing precisionVSDuration of action of stationary object

Solution Approach 1:

The patent creates a composite system where polycarboxylic acid-based copolymer provides strong dispersibility through its three-dimensional molecular structure and steric hindrance repulsion, while layered double hydroxide contributes to sustained workability maintenance. The synergistic interaction between these two components resolves the trade-off, allowing high dispersibility to be achieved without sacrificing workability maintenance.

Inventive Principle:
Principle #40Composite materials

3Reliability

If conventional PCA-based admixtures are used to reduce chloride ion infiltration, then corrosion resistance is improved, but dispersibility and workability maintenance become insufficient

Engineering Contradiction:
Improvecorrosion resistanceVSAvoiddispersibility
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent develops a composite cement admixture combining polycarboxylic acid-based copolymer with layered double hydroxide. The copolymer component ensures excellent dispersibility and workability maintenance, while the layered double hydroxide provides enhanced corrosion resistance by forming a protective barrier that reduces chloride ion infiltration. This composite structure achieves all three performance requirements simultaneously.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent applies different functional components to different aspects of concrete performance: the polycarboxylic acid-based copolymer is optimized for dispersibility and workability maintenance, while the layered double hydroxide is specifically designed to provide corrosion resistance. Each component performs its specialized function locally, and their combination achieves comprehensive performance improvement.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting cement admixture exhibits improved dispersibility, workability maintenance, and corrosion resistance, with a simplified and cost-effective manufacturing process, effectively addressing the trade-off issues of conventional PCA-based admixtures.

Implementation Method 1

The PCA-based admixtures may form a three-dimensional molecular structure due to a polyethylene oxide side chain contained in the polymer strucure, and steric hindrance repulsion caused thereby disperses cement particles, thereby fluidizing a cement composition.

Methodology Applied
Scientific EffectSteric hindrance repulsion:

Implementation Method 2

with the construction of marine concrete structures and use of washed sand, chloride ions infiltrate into the concrete structures, thereby causing corrosion in the concrete structures

Methodology Applied
Scientific EffectIon repulsion: Ion Repulsion/Attraction

Data Source

PatentEP3006423B1Cement admixture comprising polycarboxylic acid copolymer, derived from a macromonomer, and layered double hydroxide and method for preparing same
Publication Date: 2020.10.21 SILKROAD C&T
  • EP3006423B1 patent drawingFigure 1
  • EP3006423B1 patent drawingFigure 2
  • EP3006423B1 patent drawingFigure 3

AI summary

Disclosed are a macromonomer for preparing a cement admixture and a method of preparing the same; a cement admixture comprising a polycarboxylic acid-based copolymer derived from the macromonomer and a layered double hydroxide; and a method of preparing the same. The polycarboxylic acid-based copolymer comprises (a) a structural unit derived from a macromonomer compound represented by Formula 1 below and (b) a structural unit derived from an acrylic monomer represented by Formula 4. The cement admixture has superior dispersibility, workability maintenance, and corrosion resistance.         [Formula 1]:     CH2=CR1-(CH2)m-O-(CH2CH2O)n-OCO-R2-COOH         [Formula 4]:     CH2=CR3-COM1