Ceramic Coated Electrode Assembly for Secondary Battery Thermal Stability

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Solution Overview

Problem

Conventional secondary batteries face thermal instability issues due to defects in the ceramic coating layer, which can lead to internal shorts, thermal decomposition, and potential fires or explosions, as the polyolefin film separator melts or contracts at high temperatures.

Innovation Solution

A ceramic coating layer with specific particle size distribution and binder properties is applied to the electrodes, eliminating the need for a polyolefin film separator and ensuring uniform coating without defects, thereby enhancing thermal stability and preventing internal shorts.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a polyolefin film separator is used to prevent electrical short between electrodes, then electrical insulation is improved, but thermal stability deteriorates because the separator melts or contracts at high temperatures

Engineering Contradiction:
Improveelectrical insulationVSAvoidthermal stability
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The invention changes the material parameter of the separator from polyolefin film to ceramic coating layer, fundamentally altering the thermal properties while maintaining electrical insulation functionality

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite ceramic coating layer composed of multiple ceramic particles (alumina, silica, zirconia, magnesia) with different properties to achieve both electrical insulation and high thermal stability simultaneously

Inventive Principle:
Principle #40Composite materials

2Temperature

If a ceramic coating layer is formed on the electrode to improve thermal stability, then thermal stability is improved, but manufacturing complexity increases due to the need for uniform coating without defects

Engineering Contradiction:
Improvethermal stabilityVSAvoidcoating process complexity
Core Design Contradiction:
TemperatureVSDevice complexity

Solution Approach 1:

The invention optimizes the viscosity parameter of the ceramic paste to a specific range (50-5000 cP) to achieve uniform coating without defects, simplifying the manufacturing process while ensuring thermal stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention applies ceramic coating selectively on the electrode surface where thermal protection is most needed, ensuring uniform coverage without excessive material usage or complex multi-layer structures

Inventive Principle:
Principle #3Local quality

3Ease of manufacture

If the ceramic coating layer contains uncoated parts, pin holes or cracks, then manufacturing is simplified, but reliability deteriorates because current concentrates at defective portions causing internal shorts

Engineering Contradiction:
Improvecoating application easeVSAvoidinternal short prevention
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The binder acts as an intermediary material that fills gaps and connects ceramic particles, ensuring complete coverage and eliminating pin holes or cracks while maintaining the ease of paste application

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The composite ceramic paste containing multiple ceramic particles and binder creates a defect-free coating layer that prevents current concentration, maintaining both manufacturing simplicity and high reliability

Inventive Principle:
Principle #40Composite materials

4Temperature

If the separator is damaged by prolonged high temperature, then thermal resistance is reduced, but harmful effects increase due to continuous melting and electrical short

Engineering Contradiction:
Improveheat resistanceVSAvoidelectrical short and thermal decomposition
Core Design Contradiction:
TemperatureVSObject-generated harmful factors

Solution Approach 1:

The invention changes the chemical composition parameter from organic polyolefin to inorganic ceramic materials, raising the decomposition temperature well above battery operating temperatures and eliminating thermal decomposition risks

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention converts the thermal weakness of polyolefin separators into a benefit by using ceramic materials that not only resist high temperatures but also actively prevent thermal runaway through their inherent thermal stability and flame resistance

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides improved thermal stability, preventing expansion of internal shorts and reducing the risk of thermal decomposition and explosions, while also improving charge/discharge rates and battery lifetime through uniform ceramic coating.

Implementation Method 1

a ceramic coating layer which is formed by coating a ceramic paste made by mixing a binder and a solvent with ceramic powder onto at least one of the cathode or anode

Methodology Applied
Scientific EffectDeposition: Deposition (physical)

Data Source

PatentEP2079121B1Electrode Assembly and Secondary Battery having the same
Publication Date: 2019.06.05 SAMSUNG SDI CO LTD
  • EP2079121B1 patent drawingFigure 1
  • EP2079121B1 patent drawingFigure 2
  • EP2079121B1 patent drawingFigure 3

AI summary

An electrode assembly of a secondary battery includes a cathode including a cathode active material layer, an anode including an anode active material layer, and a ceramic coating layer formed on at least one of surfaces of the cathode and anode that face each other. The ceramic coating layer includes a ceramic powder and a binder. The specific surface area of the ceramic powder is more than 1.5m2/g and less than 15.0m2/g, and, in the particle size distribution of the ceramic powder, the D10 value is more than 0.05 µm and the D90 value is less than 3.0 µm.