Ceramic Hollow Microsphere Barrier Coating

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Solution Overview

Problem

Existing ceramic thermal barrier coatings are not well-suited for ceramic components due to mismatched coefficients of thermal expansion and high thermal conductivity, which can lead to spallation and microcracking when exposed to high-temperature gases.

Innovation Solution

A thermal and environmental barrier coating composed of ceramic hollow microspheres with a high void volume fraction and closed porosity, sintered together with a binder or embedded in a matrix, providing low thermal conductivity and matching the coefficient of thermal expansion of the ceramic substrate.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If traditional ceramic thermal barrier coatings are applied to ceramic substrates, then thermal protection is provided, but thermal stresses cause spallation and microcracking due to mismatched coefficients of thermal expansion

Engineering Contradiction:
Improvecoating durabilityVSAvoidthermal stress
Core Design Contradiction:
ReliabilityVSStress or pressure

Solution Approach 1:

The patent changes the physical and chemical parameters of the coating material by incorporating hollow microspheres, which fundamentally alters the coefficient of thermal expansion to match the ceramic substrate. This parameter change eliminates the thermal stress mismatch that causes spallation and microcracking in traditional coatings.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite materials by combining hollow microspheres with binder materials to create a coating with tailored thermal expansion properties. The composite structure allows the coating to match the substrate's coefficient of thermal expansion while maintaining thermal barrier functionality.

Inventive Principle:
Principle #40Composite materials

2Temperature

If traditional ceramic thermal barrier coatings are used, then thermal protection is achieved, but thermal conductivity remains high leading to heat flow into the metal component

Engineering Contradiction:
Improvethermal conductivityVSAvoidheat flow
Core Design Contradiction:
TemperatureVSLoss of energy

Solution Approach 1:

The patent employs porous materials by incorporating hollow microspheres with high void volume fractions (60-95%) into the coating. The air-filled hollow spaces act as thermal insulators, dramatically reducing thermal conductivity and minimizing heat flow to the underlying substrate.

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent changes the thermal conductivity parameter by introducing hollow microspheres with low thermal conductivity into the coating matrix. This fundamentally alters the heat transfer properties, reducing thermal conductivity from typical values of 0.8-1.6 W/mK to significantly lower values.

Inventive Principle:
Principle #35Parameter changes

3Temperature

If hollow microspheres with high void volume fraction are used to reduce thermal conductivity, then thermal insulation is improved, but coating density decreases

Engineering Contradiction:
Improvethermal conductivityVSAvoidcoating density
Core Design Contradiction:
TemperatureVSVolume of stationary object

Solution Approach 1:

The patent intentionally uses porous materials with high void volume fractions (60-95%) to achieve superior thermal insulation. The hollow microspheres create a lightweight, low-density structure that maximizes thermal resistance while maintaining coating integrity through the binder material.

Inventive Principle:
Principle #31Porous materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The coating achieves significantly reduced thermal conductivity and improved cyclic durability by minimizing thermal stresses and matching the thermal expansion of the ceramic substrate, while maintaining high temperature capability and resistance to water vapor corrosion.

Implementation Method 1

The thermal and environmental barrier coating may have low conductivity as a result of including the hollow microspheres

Methodology Applied
Scientific EffectThermal insulation: Thermal Insulation

Implementation Method 2

with a low coefficient of thermal expansion similar to the ceramic substrate

Methodology Applied
Scientific EffectThermal expansion: Thermal Expansion

Implementation Method 3

the microspheres are sintered together with a powder of another material that acts as a binder

Methodology Applied
Scientific EffectSintering: Sintering

Data Source

PatentEP3274317B1Thermal and environmental barrier coating for ceramic substrates
Publication Date: 2024.12.18 HRL LAB
  • EP3274317B1 patent drawingFigure 1A~1E
  • EP3274317B1 patent drawingFigure 2A~2C
  • EP3274317B1 patent drawingFigure 3A~3C

AI summary

A thermal and environmental barrier coating composed of ceramic hollow microspheres sintered together. In one embodiment the microspheres are sintered together with a powder of another material that acts as a binder, or with a powder of a material that may be the same as the material of the hollow microspheres, forming a matrix in which the hollow microspheres are embedded. The hollow microspheres may be composed of a material with a high temperature capability, and with a low coefficient of thermal expansion.