Ceria-Coated CMP Slurry for STI Trench Dishing Control

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Solution Overview

Problem

Existing Shallow Trench Isolation (STI) chemical mechanical polishing compositions fail to effectively reduce oxide trench dishing and achieve uniformity across various sized oxide trench features while maintaining high selectivity for silicon dioxide over silicon nitride, leading to potential electrical issues and device failure.

Innovation Solution

A chemical mechanical polishing composition using ceria-coated inorganic oxide particles combined with specific chemical additives, such as organic carboxylic acid molecules, carboxylate salts, or carboxylic ester molecules with multiple hydroxyl functional groups, which suppress SiN film removal rates and reduce oxide trench dishing, applied across a wide pH range including acidic, neutral, and alkaline conditions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional STI CMP compositions are used, then silicon dioxide removal rate is maintained, but oxide trench dishing is severe and non-uniform

Engineering Contradiction:
Improveoxide trench dishing uniformityVSAvoidtransistor isolation quality
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the CMP slurry by incorporating specific organic acids (polyacrylic acid, polymethacrylic acid, polyacrylic acid-co-maleic acid) and controlling pH levels (9-11) to modify the chemical interaction between slurry and oxide trench surfaces, reducing dishing while maintaining removal rates

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses composite abrasive systems combining ceria particles with organic acid additives, creating a multi-functional slurry that simultaneously provides mechanical abrasion and chemical etching effects to achieve uniform trench planarization

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If high oxide vs nitride selectivity is achieved, then silicon nitride removal is suppressed, but oxide trench dishing increases

Engineering Contradiction:
Improveoxide to nitride selectivityVSAvoidtrench oxide loss uniformity
Core Design Contradiction:
Manufacturing precisionVSShape

Solution Approach 1:

The patent applies different chemical mechanisms to different regions: organic acids selectively interact with oxide surfaces in trenches to reduce dishing, while the slurry maintains high selectivity for oxide over nitride removal through controlled chemical affinity and pH conditions

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

Organic acid molecules act as intermediaries that mediate between the abrasive particles and the oxide surface, modifying the chemical interaction to reduce excessive oxide removal in trenches while maintaining overall selectivity

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If polyacrylic acid is used to reduce oxide trench dishing, then dishing is reduced, but molecular weight control becomes critical for optimal performance

Engineering Contradiction:
Improveoxide trench dishing reductionVSAvoidpolymer molecular weight specification
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent specifies precise molecular weight ranges (300-20,000 for polyacrylic acid, 500-50,000 for polymethacrylic acid) to optimize the balance between dishing reduction effectiveness and slurry stability, recognizing that polymer chain length directly impacts interaction with oxide surfaces

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition achieves reduced oxide trench dishing, improved uniformity, and high oxide to nitride selectivity, preventing electrical current leakage and enhancing transistor performance by effectively suppressing SiN removal rates and maintaining high TEOS film removal rates.

Implementation Method 1

The slurry comprises cerium oxide particles and polymeric electrolyte

Methodology Applied
Scientific EffectAbrasion: Abrasion

Implementation Method 2

chemical mechanical polishing compositions containing abrasive particles and exhibiting normal stress effects

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 3

non-polishing particles resulting in reduced polishing rate at recesses

Methodology Applied
Scientific EffectChemical adsorption: Adsorption

Implementation Method 4

polymeric electrolyte... salts of polyacrylic acid

Methodology Applied
Scientific EffectElectrostatic interaction: Electrostatic Induction

Implementation Method 5

a compound which complexes with the silica and silicon nitride wherein the complexing agent has two or more functional groups each having a dissociable proton

Methodology Applied
Scientific EffectComplexation: Chemical Bonding

Implementation Method 6

an aqueous medium... pH of 4 to 9

Methodology Applied
Scientific EffectIon dissociation: Electrolysis

Implementation Method 7

aqueous medium, and an organic polyol that does not dissociate protons

Methodology Applied
Scientific EffectDiffusion: Diffusion

Data Source

PatentEP3628713B1High oxide vs nitride selectivity, low and uniform oxide trench dishing in shallow trench isolation (STI) chemical mechanical planarization polishing (CMP)
Publication Date: 2022.01.12 VERSUM MATERIALS US LLC
  • EP3628713B1 patent drawingFigure 1
  • EP3628713B1 patent drawingFigure 2
  • EP3628713B1 patent drawingFigure 3

AI summary

Present invention provides Chemical Mechanical Planarization Polishing(CMP) compositions for Shallow Trench Isolation(STI) applications. The CMP compositions contain ceria coated inorganic oxide particles as abrasives, such as ceria-coated silica particles or any other ceria-coated inorganic metal oxide particles as core particles; suitable chemical additives comprising at least one organic carboxylic acid group, at least one carboxylate salt group or at least one carboxylic ester group and two or more hydroxyl functional groups in the same molecule; and a water soluble solvent; and optionally biocide and pH adjuster; wherein the composition has a pH of 2 to 12, preferably 3 to 10, and more preferably 4 to 9.