Chromium Catalyst Composition for Consistent Flow Index

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Solution Overview

Problem

Chromium-based catalysts used in polyolefin manufacture often produce polymers with inconsistent flow index responses, leading to variations in molecular weight and processing characteristics, which can result in operational difficulties and suboptimal polymer properties for specific applications.

Innovation Solution

A chromium-based catalyst composition is developed, comprising an inorganic oxide-supported chromium catalyst, a particulate material with an average particle size of less than 5 microns, and/or an antistatic agent, which minimizes particle aggregation and improves dispersion, resulting in consistent flow index responses and enhanced polymer properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If chromium oxide-on-silica catalysts are used, then productivity is improved, but molecular weight distribution becomes narrower

Engineering Contradiction:
ImproveproductivityVSAvoidmolecular weight distribution
Core Design Contradiction:
ProductivityVSStability of the object's composition

Solution Approach 1:

An organometallic compound (intermediary substance) is introduced to modify the chromium-based catalyst, creating a new catalyst system that combines the high productivity of chromium oxide-on-silica with the ability to produce broader molecular weight distributions suitable for blow molding applications

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The catalyst system parameters are changed by adding organometallic compounds and adjusting preparation conditions (drying temperature, reducing agent addition time) to achieve both high productivity and desirable molecular weight distribution characteristics

Inventive Principle:
Principle #35Parameter changes

2Stability of the object's composition

If silyl chromate-based catalysts are used, then molecular weight characteristics are improved, but productivity decreases

Engineering Contradiction:
Improvemolecular weight distributionVSAvoidproductivity
Core Design Contradiction:
Stability of the object's compositionVSProductivity

Solution Approach 1:

The invention merges the advantages of silyl chromate catalysts (broad molecular weight distribution) with chromium oxide-on-silica catalysts (high productivity) by using organometallic compounds to modify the chromium-based catalyst system, achieving both desired molecular weight characteristics and high productivity

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

A composite catalyst system is created by combining chromium-based catalyst components with organometallic compounds, resulting in a catalyst that exhibits both high productivity and broad molecular weight distribution suitable for blow molding applications

Inventive Principle:
Principle #40Composite materials

3Productivity

If chromium-based catalysts are used, then polyolefin production is achieved, but flow index response varies between batches

Engineering Contradiction:
Improvepolymer productionVSAvoidflow index consistency
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The invention establishes controlled preparation procedures with specific parameters (drying temperature ranges, reducing agent addition times, organometallic compound ratios) that provide feedback control over catalyst properties, ensuring consistent flow index responses across batches

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The catalyst preparation includes preliminary steps (drying at controlled temperatures, controlled addition of reducing agents and organometallic compounds) that pre-establish consistent catalyst properties before polymerization, reducing batch-to-batch variation in flow index responses

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalyst composition achieves improved homogeneity and batch-to-batch consistency, reducing variations in flow index responses and enabling the production of polymers with desired molecular weight ranges, thus facilitating the production of polyolefins with specific properties for various applications.

Implementation Method 1

heated in the presence of oxygen to about 400° C.-860° C., converting most or all of the chromium from the +3 to the +6 oxidation state

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

contacting the activated chromium-based catalyst with an organometallic compound

Methodology Applied
Scientific EffectReduction: Reduction

Data Source

PatentUS10266618B2Chromium-based catalyst compositions for olefin polymerization
Publication Date: 2019.04.23 UNIVATION TECH LLC

AI summary

Modified chromium-based catalyst compositions for olefin polymerization are disclosed. The modifiers prevent or reduce catalyst particle aggregation providing improved catalyst particle dispersion and consistent flow index response of the compositions in olefin polymerization.