Chromium Catalyst Composition for Consistent Flow Index

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Solution Overview

Problem

Chromium-based catalysts used in polyolefin manufacture often produce polymers with inconsistent flow index responses, leading to variations in molecular weight and processing characteristics, which can result in operational difficulties and undesirable polymer properties.

Innovation Solution

A chromium-based catalyst composition is developed, comprising thermally treated particulate material with chromium compounds, aluminium alkyl species, and a hydrophobic particulate material like treated fumed silica, which minimizes particle agglomeration and improves dispersion, thereby enhancing batch consistency and reducing flow index variation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If chromium oxide-on-silica catalysts are used, then productivity is improved, but molecular weight distribution becomes narrower than desired

Engineering Contradiction:
ImproveproductivityVSAvoidmolecular weight distribution
Core Design Contradiction:
ProductivityVSStability of the object's composition

Solution Approach 1:

The patent combines chromium oxide-on-silica catalyst (providing high productivity) with silyl chromate catalyst (providing desirable molecular weight distribution characteristics) into a single composite catalyst system, thereby achieving both high productivity and broad molecular weight distribution simultaneously

Inventive Principle:
Principle #5Merging (Combining)

2Stability of the object's composition

If silyl chromate-based catalysts are used, then molecular weight distribution becomes broader, but productivity decreases

Engineering Contradiction:
Improvemolecular weight distributionVSAvoidproductivity
Core Design Contradiction:
Stability of the object's compositionVSProductivity

Solution Approach 1:

The patent combines chromium oxide-on-silica catalyst (providing high productivity) with silyl chromate catalyst (providing desirable molecular weight distribution characteristics) into a single composite catalyst system, thereby achieving both high productivity and broad molecular weight distribution simultaneously

Inventive Principle:
Principle #5Merging (Combining)

3Productivity

If chromium-based catalysts are used without modification, then catalytic activity is maintained, but flow index response becomes inconsistent

Engineering Contradiction:
Improvecatalytic activityVSAvoidflow index consistency
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent introduces a reducing agent as an intermediary substance that modifies the chromium-based catalyst surface, creating intermediate species that provide consistent flow index response while maintaining high catalytic activity for polyolefin production

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalyst composition achieves consistent flow index responses, improving the homogeneity and bulk density of the catalyst, leading to more reliable polymer production with desired properties, such as higher molecular weight and improved processing characteristics.

Implementation Method 1

The thermally treated particulate material is treated at an elevated temperature to convert chromium atoms into the +6 state and/or to remove moisture

Methodology Applied
Scientific EffectThermal treatment: Heat Treatment

Implementation Method 2

treating the thermally treated particulate material with a reducing agent

Methodology Applied
Scientific EffectRedox reactions: Redox Reactions

Data Source

PatentEP3223943B1Composition comprising particles
Publication Date: 2023.09.27 UNIVATION TECH LLC

AI summary

Modified chromium-based catalyst compositions for olefin polymerization are disclosed. The modifiers prevent or reduce catalyst particle aggregation providing improved catalyst particle dispersion and consistent flow index response of the compositions in olefin polymerization.