CMP Composition for Selective Titanium Nitride and Titanium Removal

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Solution Overview

Problem

There is a need for enhanced chemical mechanical polishing compositions that exhibit improved tungsten polishing rates and selective removal rates between titanium nitride and titanium features, as existing methods lack sufficient selectivity and efficiency in planarizing semiconductor substrates.

Innovation Solution

A chemical mechanical polishing composition comprising water, an oxidizing agent, a linear polyalkylenimine polymer, a colloidal silica abrasive with a positive surface charge, a carboxylic acid, and a source of ferric ions, with a pH of 1 to 4, is used in conjunction with a polishing pad to create dynamic contact, enabling selective removal of titanium nitride and titanium features with a removal rate selectivity of ≥100.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional polishing compositions are used, then titanium nitride can be removed, but titanium is also removed at a high rate reducing selectivity

Engineering Contradiction:
Improveselectivity between titanium nitride and titanium removalVSAvoidtitanium removal rate
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The polishing composition uses a highly acidic pH range (1-4) with specific buffering agents to control the chemical environment. This parameter change enables selective oxidation and removal of titanium nitride while protecting titanium, achieving ≥100:1 selectivity through controlled chemical reactions rather than mechanical abrasion alone

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

Organic buffering agents and complexing agents act as intermediaries that selectively interact with titanium nitride surfaces. These additives mediate the chemical reactions by forming temporary complexes with titanium nitride, facilitating selective removal while leaving titanium intact through controlled chemical pathways

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If polishing pressure and speed are increased to improve planarization rate, then tungsten and titanium nitride removal rate increases, but control over selective removal becomes difficult

Engineering Contradiction:
Improveplanarization rateVSAvoidselective removal control
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The invention replaces reliance on mechanical polishing parameters (pressure, speed) with a chemically-driven process. The highly acidic composition with specific additives performs the bulk of the removal work through chemical oxidation and dissolution, allowing mechanical parameters to be optimized for selectivity rather than just removal rate

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

By changing the chemical composition parameters (pH 1-4, specific buffering agents, complexing agents), the process achieves high planarization rates through enhanced chemical reactivity. This allows decoupling of productivity from mechanical intensity, maintaining selectivity while improving overall removal rate through chemical enhancement

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition achieves rapid removal of tungsten and titanium nitride while significantly reducing titanium removal, thereby enhancing planarization efficiency and selectivity, particularly in semiconductor substrates with exposed titanium nitride and titanium features.

Implementation Method 1

a colloidal silica abrasive with a positive surface charge

Methodology Applied
Scientific EffectAbrasion: Abrasion

Implementation Method 2

an oxidizing agent

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentUS10573524B2Method of chemical mechanical polishing a semiconductor substrate
Publication Date: 2020.02.25 RODEL HLDG INC

AI summary

A process for chemical mechanical polishing a substrate containing titanium nitride and titanium is provided comprising: providing a polishing composition, containing, as initial components: water; an oxidizing agent; a linear polyalkylenimine polymer; a colloidal silica abrasive with a positive surface charge; a carboxylic acid; a source of ferric ions; and, optionally pH adjusting agent; wherein the polishing composition has a pH of 1 to 4; providing a chemical mechanical polishing pad, having a polishing surface; creating dynamic contact at an interface between the polishing pad and the substrate; and dispensing the polishing composition onto the polishing surface at or near the interface between the polishing pad and the substrate; wherein at least some of the titanium nitride and at least some of the titanium is polished away with a selectivity between titanium nitride and titanium.