Carbon Nanotube Immobilization via Linking Groups for Peel Resistance

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Conventional transparent conductive films using carbon nanotubes face issues with insufficient adhesion to base materials, leading to peeling, and struggle to achieve both high light transmittance and conductivity due to structural limitations and defects.

Innovation Solution

A method involving chemical bonding of carbon nanotubes to a base material surface using linking groups such as -NH, -NH-R1-NH, -SO, R2, or -O-R3 groups, facilitated by surface modifications with functional groups like -NH2, -NH-R1-NH2, -SOCl, -R2-MgX, -O-R3-ONa, and -R2-Li, enhances adhesion and stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If carbon nanotubes are used to form transparent conductive films, then conductivity and light transmittance are improved, but adhesion to base material deteriorates causing peeling

Engineering Contradiction:
Improveconductivity and light transmittanceVSAvoidadhesion to base material
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent introduces a silane-based linking group as an intermediary between the carbon nanotubes and the base material. This linking group forms chemical bonds with both the carbon nanotubes and the base material, acting as a bridge that transfers adhesion forces and prevents peeling while maintaining the electrical and optical properties of the carbon nanotube film.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite structure consisting of carbon nanotubes, silane-based linking groups, and base material. This composite approach combines the advantages of carbon nanotubes (conductivity, transparency) with the adhesion benefits of silane chemistry, resulting in a multi-functional material system that resolves the contradiction between film properties and adhesion.

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If multi-walled carbon nanotubes with small aspect ratio are used, then production cost is reduced, but light transmittance and conductivity deteriorate

Engineering Contradiction:
Improveproduction costVSAvoidlight transmittance and conductivity
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent changes the structural parameters of the carbon nanotubes by introducing silane-based functional groups at specific positions along the nanotube structure. This modification allows the use of shorter, more cost-effective carbon nanotubes while maintaining excellent electrical and optical properties through the enhanced interfacial bonding provided by the silane linking groups.

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If carbon nanotubes are simply laminated on base material, then ease of manufacture is improved, but adhesion deteriorates leading to peeling

Engineering Contradiction:
Improveease of manufactureVSAvoidadhesion
Core Design Contradiction:
Ease of manufactureVSStrength

Solution Approach 1:

The patent applies silane-based functional groups to the carbon nanotubes before forming the final film structure. This preliminary functionalization ensures that adhesion capabilities are built into the nanotube structure itself, allowing for simple lamination processes while guaranteeing strong bonding to the base material through the pre-installed silane linking groups.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The immobilized carbon nanotubes provide improved resistance to peeling and enable functionalities like conductivity, electrical static dissipative, and antistatic properties with long-term stability.

Implementation Method 1

the carbon nanotube is chemically bonded on the base material surface via a linking group

Methodology Applied
Scientific EffectChemical bonding: Chemical Bonding

Implementation Method 2

the linking group is formed via a chemical bond between a fluorine group on a surface of the carbon nanotube before immobilizing and an amino group on the base material

Methodology Applied
Scientific EffectAmide bond formation: Chemical Bonding

Data Source

PatentEP3451349B1Immobilized product and method for producing same
Publication Date: 2025.11.12 STELLA CHEMIFA CORP
  • EP3451349B1 patent drawingFigure 1
  • EP3451349B1 patent drawingFigure 2

AI summary

To provide a novel immobilized product in which a carbon material and/or a silicon material is/are immobilized on a base material surface by a chemical bond via a linking group, and a method for producing the same. The immobilized product (10) of the present invention is an immobilized product in which a carbon material (11) is immobilizing on a surface of a base material (12), wherein the carbon material (11) is chemically bonded on the surface of the base material (12) via a linking group, and the linking group is at least any one selected from the group consisting of a -NH group, a -NH-R1-NH group, a -SO group, a R2 group, an -O-R3-O group, and a R4 group (in which the R1 to R4 each independently represent at least one selected from the group consisting of a chain alkyl group, a cyclic alkyl group, a chain alkenyl group, a cyclic alkenyl group, a chain alkynyl group, an aryl group, and functional groups in which at least one of a hydroxyl group, a halogen, an ester group, an ether group, a carbonyl group, an amino group, an amide group, a cyano group, a thiol group, a thioester group, or a thioether group is further bonded to these functional groups).