Coated Natural Graphite for Battery Electrodes

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current carbon materials for lithium ion secondary batteries face challenges in achieving high energy density, long cycle life, and large current load characteristics, particularly for applications requiring ultralong-term cycle characteristics and high power output, such as electric vehicles.

Innovation Solution

A carbon material with specific structural and chemical properties, including a Raman spectroscopy ratio of 0.38 to 1.2, an average interplanar spacing of 0.335 to 0.338 nm, and a BET specific surface area of 2 to 25 m^2/g, produced through a process involving calcined coke heat treatment and mixing with petroleum pitch, is used to enhance lithium ion diffusion and electrode density.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If natural graphite is used as negative electrode active material, then cost is reduced, but alignment occurs during electrode production which degrades electrode performance

Engineering Contradiction:
ImprovecostVSAvoidelectrode performance
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent uses composite materials by coating artificial carbon on the surface of natural graphite particles. This composite structure combines the cost advantage of natural graphite with the performance benefits of artificial carbon, preventing alignment and maintaining electrode performance while keeping costs low.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent changes the surface properties of natural graphite by coating it with artificial carbon, modifying parameters such as surface roughness, conductivity, and structural stability. This prevents the alignment issue during electrode production while maintaining the cost benefits of natural graphite.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If natural graphite is granulated and formed into spherical shape, then alignment is reduced, but surface activity increases causing gas generation and decreased initial efficiency

Engineering Contradiction:
Improvealignment resistanceVSAvoidgas generation
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent modifies the surface parameters of spherical natural graphite by coating it with artificial carbon. This reduces surface activity and prevents gas generation during initial charging, while maintaining the alignment resistance provided by the spherical shape.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent converts the harmful surface activity of natural graphite into a benefit by coating it with artificial carbon. The coating material reacts with the surface to form a stable structure that prevents gas generation, turning the initially harmful surface activity into a controlled process that improves overall battery performance.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Productivity

If artificial graphite with highly-developed fine pores is used, then high-rate discharge is improved, but manufacturing complexity increases

Engineering Contradiction:
Improvehigh-rate dischargeVSAvoidmanufacturing complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent uses porous artificial carbon material to coat the natural graphite particles. The porous structure provides highly-developed fine pores that enable high-rate discharge, while the coating process itself is a relatively simple manufacturing step that can be integrated into existing production lines.

Inventive Principle:
Principle #31Porous materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The carbon material improves lithium ion diffusion, leading to high energy density, high-speed charge and discharge capabilities, while maintaining high capacity and cycle characteristics, and is produced with economic efficiency and improved safety.

Implementation Method 1

the carbon material improves lithium ion diffusion, leading to high energy density, high-speed charge and discharge capabilities

Methodology Applied
Scientific EffectLithium ion diffusion: Diffusion

Implementation Method 2

produced through a process involving calcined coke heat treatment and mixing with petroleum pitch

Methodology Applied
Scientific EffectHeat treatment: Heat Treatment

Data Source

PatentUS10377634B2Carbon material, material for a battery electrode, and battery
Publication Date: 2019.08.13 RESONAC CORP

AI summary

A carbon material and a material for a battery electrode which is suitable for use as an electrode material for an aqueous-electrolyte secondary battery, which material includes optical structures having a specific shape, and in which material the ratio IG/ID (R value) between the peak intensity (ID) of a peak in a range of 1300 to 1400 cm−1 and the peak intensity (IG) of a peak in a range of 1580 to 1620 cm−1 measured by Raman spectroscopy spectra when particles of the carbon material are measured with Raman microspectrometer is 0.38 or more and 1.2 or less and the average interplanar spacing d002 of plane (002) by the X-ray diffraction method is 0.335 nm or more and 0.338 nm or less; and a secondary battery excellent in charge/discharge cycle characteristics and large current load characteristics.