Two-Stage Combustion NOx Reduction via Calorific Value Control

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Solution Overview

Problem

Current combustion processes in technical furnaces, such as grate furnaces, face challenges in reducing nitrogen oxide (NOx) formation while avoiding the formation of nitrous oxide (N2O) and ammonia slip (NH3), which are not effectively addressed by existing methods that either lead to incomplete combustion or reduce heat energy utilization.

Innovation Solution

A method involving a two-stage combustion process with a fixed bed burnout zone and a downstream exhaust gas burnout zone, where a gas-water mixture is injected to reduce the calorific value of exhaust gases before the exhaust gas burnout zone, maintaining temperatures above 950°C to prevent N2O formation and ensuring complete breakdown of NH3, while adjusting primary air supply and grate kinematics to optimize combustion stoichiometry and gas mixing.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-generated harmful factors

If the calorific value of exhaust gases is reduced before the exhaust gas burnout zone, then NOx emissions are reduced, but the temperature may drop below 950°C causing N2O formation

Engineering Contradiction:
ImproveNOx emissionsVSAvoidexhaust gas temperature
Core Design Contradiction:
Object-generated harmful factorsVSTemperature

Solution Approach 1:

The patent applies parameter changes by precisely controlling the calorific value of exhaust gases within a specific range (0.3-1.5 MJ/m³) before the exhaust gas burnout zone. This controlled parameter change reduces NOx formation while maintaining sufficient temperature (>950°C) to prevent N2O formation, resolving the contradiction between reducing harmful emissions and maintaining temperature.

Inventive Principle:
Principle #35Parameter changes

2Productivity

If secondary air is added to complete exhaust gas burnout, then combustion efficiency is improved, but local temperature peaks increase causing NOx formation

Engineering Contradiction:
Improvecombustion efficiencyVSAvoidNOx formation
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent applies local quality by creating different oxygen concentration zones: the primary combustion zone operates with controlled oxygen supply to limit temperature peaks and NOx formation, while the exhaust gas burnout zone receives additional secondary air specifically for completing the burnout of remaining combustible gases. This localized differentiation of combustion conditions achieves both complete combustion efficiency and NOx reduction.

Inventive Principle:
Principle #3Local quality

3Object-generated harmful factors

If primary air supply is increased to reduce NOx, then nitrogen oxide formation is reduced, but heat energy utilization decreases

Engineering Contradiction:
ImproveNOx formationVSAvoidheat energy utilization
Core Design Contradiction:
Object-generated harmful factorsVSLoss of energy

Solution Approach 1:

The patent applies preliminary action by pre-cooling and pre-mixing the exhaust gases before they enter the exhaust gas burnout zone. This preliminary preparation reduces the calorific value to an optimal range, allowing subsequent complete burnout with secondary air to proceed at controlled temperatures that minimize NOx formation while maximizing heat energy recovery from the exhaust gases.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly reduces NOx emissions without forming N2O or causing ammonia slip, maintains high heat energy utilization, and ensures good slag quality by controlling the calorific value and temperature of exhaust gases, thereby meeting stringent emission limits and operational efficiency.

Implementation Method 1

a gas-water mixture is injected to reduce the calorific value of exhaust gases before the exhaust gas burnout zone

Methodology Applied
Scientific EffectEvaporative cooling: Evaporative Cooler

Implementation Method 2

a gas-water mixture is injected to reduce the calorific value of exhaust gases

Methodology Applied
Scientific EffectPhase change: Phase Change

Implementation Method 3

the primary nitrogen species NH 3 and HCN are completely broken down and N 2 is preferably formed as the end product

Methodology Applied
Scientific EffectCombustion: Combustion

Implementation Method 4

the primary nitrogen species NH 3 and HCN are completely broken down and N 2 is preferably formed as the end product at the expense of nitrogen oxide formation

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 5

maintaining temperatures above 950°C to prevent N2O formation and ensuring complete breakdown of NH3

Methodology Applied
Scientific EffectThermal decomposition: Thermolysis

Data Source

PatentEP1982112B1Method of reducing nitrogen oxide on the primary side in a two-stage combustion process
Publication Date: 2017.09.13 KARLSRUHER INST FUR TECH
  • EP1982112B1 patent drawingFigure 1
  • EP1982112B1 patent drawingFigure 2a~2f
  • EP1982112B1 patent drawingFigure 3a

AI summary

Method of reducing the nitrogen oxide formation (NOx) on the primary side and of at the same time avoiding the formation of nitrous oxide (N2O) and ammonia slip (NH3) in the exhaust gas of a two-stage combustion process and of improving the slag balance, comprising a fixed-bed burn-out zone, through which an oxygenous primary gas flows, above a fuel bed and a downstream exhaust-gas burn-out zone into which oxygenous secondary gas is additionally introduced. The object is to propose a simple and reliably controllable method for reducing nitrogen oxide formation on the primary side in combustion plants, for example grate combustion plants, with considerably higher efficiency, wherein no additional pollutants are produced or the utilization of the energy of the heat content of the combustion gases is only marginally impaired. The object is achieved in that the calorific value of the exhaust gas between the fuel bed surface and upstream of the exhaust-gas burn-out zone is reduced in such a way that an average calorific value of less than 1 MJ/m3 occurs, and the temperature of the fuel bed surface is at least 950°C until the exhaust gas leaves the exhaust-gas burn-out zone, and the gas temperature above the fuel bed in the region of the rear grate half is more than 1000°C.