Lithium Complex Soap Grease Processing in Non-Polar Base Oils

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Solution Overview

Problem

Conventional processes for producing lithium complex soap lubricating greases face challenges in achieving high dropping points, especially when using non-polar base oils, due to the lack of complex soap associations, and require excessive lithium hydroxide, which may be hazardous and costly.

Innovation Solution

Saponifying dicarboxylic acids with lithium or calcium hydroxide in a solid form in an aqueous environment, followed by reaction with hydroxy fatty acids and additional metal hydroxides, allowing for the formation of lithium or calcium complex soaps in an oleophilic base oil, thereby enhancing dropping points and reducing raw material usage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If saponification is carried out directly in base oil, then the process is simpler, but the dropping point remains low due to lack of complex soap associations

Engineering Contradiction:
Improveprocess simplicityVSAvoiddropping point
Core Design Contradiction:
Ease of manufactureVSTemperature

Solution Approach 1:

The saponification process is divided into two separate stages: first saponifying dicarboxylic acid with metal hydroxide in aqueous medium to form metal salt, then reacting this salt with hydroxy fatty acid in base oil to form complex soap. This segmentation allows formation of the desired complex soap structure that achieves high dropping points while maintaining process feasibility.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The dicarboxylic acid is saponified in advance in an aqueous environment to form the metal salt before introducing it to the base oil system. This preliminary action ensures that the complex soap associations can form properly in the base oil, achieving the required dropping point without compromising process simplicity.

Inventive Principle:
Principle #10Preliminary action

2Reliability

If excessive lithium hydroxide is used to ensure complete saponification, then the reaction completeness improves, but safety and cost worsen

Engineering Contradiction:
Improvereaction completenessVSAvoidsafety hazards
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The metal salt of dicarboxylic acid serves as an intermediary that facilitates complete saponification of hydroxy fatty acid with stoichiometric amounts of lithium hydroxide. This intermediary approach ensures reaction completeness while avoiding the need for excessive lithium hydroxide, thereby improving safety and reducing costs.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The process changes the form of metal hydroxide from aqueous solution to solid form, and introduces the metal salt of dicarboxylic acid as an intermediate compound. This parameter change allows for more precise control of lithium hydroxide dosage, ensuring complete reaction without excess, thus improving safety and cost-effectiveness.

Inventive Principle:
Principle #35Parameter changes

3Stability of the object's composition

If non-polar base oils are used, then the grease has good stability, but the dropping point decreases due to lack of complex soap formation

Engineering Contradiction:
Improvegrease stabilityVSAvoiddropping point
Core Design Contradiction:
Stability of the object's compositionVSTemperature

Solution Approach 1:

The process introduces a two-stage approach with intermediate metal salt formation, which enables complex soap structure formation even in non-polar base oils. This parameter change in the reaction pathway allows maintaining grease stability while achieving high dropping points through proper complex soap associations.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves high dropping points above 260°C for lithium complex soap greases and 190°C for calcium-lithium complex soap greases, improving thickener yield, mechanical stability, and reducing lithium hydroxide usage, while being more energy-efficient and safer.

Implementation Method 1

Saponifying dicarboxylic acids with lithium or calcium hydroxide in a solid form in an aqueous environment

Methodology Applied
Scientific EffectSaponification: Hydrolysis

Implementation Method 2

bringing into contact with one or more liquid or liquefied by heating hydroxy fatty acids and dissolving the metal salt(s) in the liquid hydroxy fatty acid

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 3

adding further metal hydroxides, wherein according to alternative: (A1) lithium hydroxide or calcium hydroxide; (A2) lithium hydroxide and calcium hydroxide or only lithium hydroxide or only calcium hydroxide; or (A3) lithium hydroxide is added; for saponification with the at least one hydroxy fatty acid

Methodology Applied
Scientific EffectSaponification: Hydrolysis

Implementation Method 4

driving off water with heating

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP4222236B1Method for producing lubricating greases of lithium complex soaps and lithium-calcium complex soaps
Publication Date: 2025.01.01 FUCHS PETROLUB AG

AI summary

The invention relates to a method for producing lubricating greases of lithium complex soaps or lithium-calcium complex soaps, to corresponding lubricating greases produced according to said method and to the use thereof in sliding and rolling bearings.