Composite Catalyst with Polymer Layer for Polyethylene Production

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Solution Overview

Problem

Existing catalyst systems struggle to produce polyethylene resins with broad molecular weight distributions in a single reactor, as they often interfere with each other, leading to unsatisfactory mechanical properties and difficulties in forming composite catalysts like Ziegler-chromium systems.

Innovation Solution

A composite catalyst is developed by separating two or more catalysts with different performances using a polymer layer, allowing for the production of polyethylene with broad molecular weight distributions and higher bulk densities, where the first catalyst is supported on a substrate, coated with a polymer layer, and the second catalyst is supported in or on this polymer layer.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If multiple catalysts are used simultaneously in a single reactor to produce polyethylene with broad molecular weight distribution, then the molecular weight distribution broadens, but the catalysts interfere with each other leading to unsatisfactory mechanical properties

Engineering Contradiction:
Improvemolecular weight distributionVSAvoidmechanical properties
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

The catalyst system is segmented into spatially separated catalyst particles (first catalyst particles and second catalyst particles) within the reactor. Each catalyst type operates independently in its own particle form, eliminating interference between catalysts while still achieving broad molecular weight distribution through physical mixing of polymers from different catalysts.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

An inert support material or spacer acts as an intermediary between different catalyst types, preventing direct interaction and interference between catalysts while allowing both to function simultaneously in the same reactor environment.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Stability of the object's composition

If Ziegler-Natta catalyst and chromium-based catalyst are used simultaneously, then broad molecular weight distribution can be achieved, but the two catalyst systems interfere with each other making it difficult to form composite catalyst

Engineering Contradiction:
Improvemolecular weight distributionVSAvoidcomposite catalyst formation
Core Design Contradiction:
Stability of the object's compositionVSEase of manufacture

Solution Approach 1:

The Ziegler-Natta catalyst and chromium-based catalyst are manufactured as separate, independent catalyst particles rather than attempting to form a composite catalyst. This segmentation avoids the interference issues that prevent composite formation while still achieving the desired broad molecular weight distribution through reactor mixing of polymers from both catalyst types.

Inventive Principle:
Principle #1Segmentation

3Stability of the object's composition

If metallocene catalyst and Ziegler-Natta catalyst are used together, then different molecular weight polymers are produced, but the mechanical properties of the resins are not satisfactory

Engineering Contradiction:
Improvemolecular weight distributionVSAvoidmechanical properties
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

The metallocene and Ziegler-Natta catalysts are used as separate catalyst particles with distinct functions. The metallocene catalyst produces low molecular weight polymer with more branched chains, while the Ziegler-Natta catalyst produces high molecular weight polymer with less branched chains. Using them as separate particles rather than mixed in a composite allows each to perform optimally, improving mechanical properties.

Inventive Principle:
Principle #1Segmentation

4Device complexity

If catalysts are physically mixed without separation, then composite catalyst can be formed, but catalyst interference occurs reducing production efficiency

Engineering Contradiction:
Improvecatalyst structureVSAvoidproduction efficiency
Core Design Contradiction:
Device complexityVSProductivity

Solution Approach 1:

Different catalyst types are segmented into separate catalyst particles rather than being physically mixed in a composite structure. This eliminates catalyst interference that reduces productivity while maintaining a relatively simple overall catalyst system structure that can be easily handled and processed.

Inventive Principle:
Principle #1Segmentation

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enables the production of polyethylene with improved mechanical and processing properties, achieving higher yield strengths and broader molecular weight distributions compared to traditional catalyst systems, while preventing catalyst interference and enhancing resin regularity and density.

Implementation Method 1

a composite catalyst useful in the production of a polyethylene, comprising at least a first catalyst and a second catalyst separated by a polymer layer

Methodology Applied
Scientific EffectPhysical separation:

Implementation Method 2

the first catalyst and the second catalyst being identical or different... a composite catalyst useful in the production of a polyethylene

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentUS8536286B2Composite catalyst for production of polyethylene
Publication Date: 2013.09.17 CHINA PETROLEUM & CHEMICAL CORP

AI summary

A composite catalyst useful in the production of polyethylene, which comprises at least a first catalyst and a second catalyst separated by a polymer layer, with the first catalyst and the second catalyst being identical or different, is described. A composite catalyst useful in the production of polyethylene with a broad molecular weight distribution in a single polymerization reactor, which comprises at least a first catalyst and a second catalyst separated by a polymer layer, with the first catalyst and the second catalyst being different, is also described. A process for preparing said catalysts and a process for the production of a polyethylene by using said catalysts are also described.