Composite Cathode Material for High-Voltage Low-Temperature Li Batteries

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Solution Overview

Problem

Existing rechargeable lithium batteries face challenges in achieving high energy density, high operating voltage, and low-temperature performance.

Innovation Solution

A positive electrode active material comprising first particles with an olivine structure and second particles with a spinel structure, where the first particles are predominant, enhancing conductivity and stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If a single-phase positive electrode active material is used, then the material structure is simple, but the energy density and operating voltage are limited

Engineering Contradiction:
Improveenergy densityVSAvoidmaterial structure complexity
Core Design Contradiction:
Quantity of substanceVSDevice complexity

Solution Approach 1:

The patent employs a composite positive electrode active material consisting of two distinct phases: an olivine phase (LiFePO4-based) and a spinel phase (LiMn2O4-based). This composite structure allows the material to simultaneously achieve high energy density from the olivine phase and high operating voltage from the spinel phase, while maintaining structural stability through the synergistic interaction between the two phases.

Inventive Principle:
Principle #40Composite materials

2Reliability

If conventional positive electrode materials are used, then the manufacturing process is simple, but the conductivity and low-temperature performance are insufficient

Engineering Contradiction:
Improvelow-temperature performanceVSAvoidmanufacturing complexity
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent optimizes the compositional parameters of the composite material, specifically controlling the molar ratio of the olivine phase to spinel phase, and adjusting the doping elements (such as Mg, Al, or Ti) to achieve optimal electrical conductivity and low-temperature performance. By precisely controlling these parameters during synthesis, the material achieves high reliability without significantly complicating the manufacturing process.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution results in a rechargeable lithium battery with improved energy density, operating voltage, and low-temperature properties.

Implementation Method 1

a positive electrode active material comprising first particles comprising a compound of Chemical Formula 1 that has an olivine structure

Methodology Applied
Scientific EffectIntercalation: Absorption (physical)

Implementation Method 2

second particles comprising a compound of Chemical Formula 2 that has a spinel structure

Methodology Applied
Scientific EffectConduction: Conduction (electrical)

Implementation Method 3

A rechargeable lithium battery produces electrical energy through the oxidation and reduction reactions when lithium ions are intercalated into and deintercalated from the positive electrode and negative electrode

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 4

A rechargeable lithium battery produces electrical energy through the oxidation and reduction reactions when lithium ions are intercalated into and deintercalated from the positive electrode and negative electrode

Methodology Applied
Scientific EffectReduction: Reduction

Data Source

PatentEP4645428A1Positive electrode active material for rechargeable lithium battery, positive electrode including the positive electrode active material, and rechargeable lithium battery including the positive electrode active material
Publication Date: 2025.11.05 SAMSUNG SDI CO LTD
  • EP4645428A1 patent drawingFigure 1
  • EP4645428A1 patent drawingFigure 2
  • EP4645428A1 patent drawingFigure 3

AI summary

A positive electrode active material comprises first particles comprising a compound having an olivine structure, and second particles comprising a compound having a spinel structure. The amount of the first particles is greater than the amount of the second particles. Also disclosed are positive electrodes including the positive electrode active materials, and rechargeable lithum batteries including the positive electrodes.