Boron-Silicon-Glass Coating to Prevent Composite Edge Oxidation

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Solution Overview

Problem

Carbon-carbon composite structures in high-temperature applications, such as aircraft braking systems, face significant oxidation issues despite existing oxidation protection systems, with phosphate-based systems experiencing viscosity decrease and migration at non-wear surface edges, and CVD-based systems being costly.

Innovation Solution

A boron-silicon-glass composite slurry is applied to the composite structure, comprising boron carbide, silicon carbide, and borosilicate glass, which forms a boron-silicon-glass layer upon heating, providing effective oxidation protection and self-healing properties without the need for chemical vapor deposition.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If phosphate-based oxidation protection systems are applied to carbon-carbon composites, then oxidation resistance is improved, but the system experiences viscosity decrease and migration at high temperatures, causing protection failure at non-wear surface edges

Engineering Contradiction:
Improveoxidation resistanceVSAvoidviscosity stability
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent modifies the chemical composition parameters of the oxidation protection system by incorporating boron carbide particles (5-20 micrometers) and boron nitride particles (5-20 micrometers) into the phosphate glass matrix. This compositional adjustment maintains high-temperature viscosity stability while preserving oxidation resistance, preventing the migration issue that plagues conventional phosphate-based systems.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If CVD process is used to apply boron carbide and silicon carbide coatings, then oxidation protection effectiveness is improved, but manufacturing cost increases significantly

Engineering Contradiction:
Improveoxidation protection effectivenessVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent replaces the expensive CVD process with a cost-effective slurry application method. The oxidation protection layer is applied as a slurry containing phosphate glass powder, boron carbide particles, and boron nitride particles, then cured at relatively low temperatures (200-400°C). This approach achieves comparable oxidation protection to CVD while dramatically reducing manufacturing costs and equipment requirements.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Object-affected harmful factors

If phosphate-based oxidation protection systems are used, then initial oxidation protection is provided, but significant oxidation of carbon-carbon composites still occurs during operation at high temperatures

Engineering Contradiction:
Improveoxidation protectionVSAvoidcarbon material loss
Core Design Contradiction:
Object-affected harmful factorsVSLoss of substance

Solution Approach 1:

The patent creates a composite oxidation protection layer by combining phosphate glass matrix with boron carbide and boron nitride particles. This composite structure provides superior oxidation resistance compared to conventional phosphate-based systems, significantly reducing carbon material loss during high-temperature operation. The boron-containing particles form protective borosilicate glass phases that effectively barrier oxygen diffusion.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The boron-silicon-glass layer significantly reduces material loss due to oxidation, offering superior protection compared to phosphate-based systems and comparable effectiveness to CVD-based systems while minimizing costs and migration issues.

Implementation Method 1

Oxidation protection system having coatings of boron carbide and silicon carbide applied via chemical vapor deposition (CVD) have demonstrated effective oxidation protection at high operating temperature.

Methodology Applied
Scientific EffectChemical Vapour Deposition: Chemical Vapour Deposition

Implementation Method 2

heating the composite structure to a temperature sufficient to form a boron-silicon-glass layer on the composite structure

Methodology Applied
Scientific EffectSintering: Sintering

Implementation Method 3

Phosphate-based oxidation protection systems may reduce infiltration of oxygen and oxidation catalysts into the composite structure.

Methodology Applied
Scientific EffectOxidation resistance: Oxidation

Data Source

PatentEP3800170A1High temperature oxidation protection for composites
Publication Date: 2021.04.07 GOODRICH CORP
  • EP3800170A1 patent drawingFigure 1A
  • EP3800170A1 patent drawingFigure 1B
  • EP3800170A1 patent drawingFigure 2

AI summary

Systems and methods for forming an oxidation protection system on a composite structure are provided. In various embodiments, an oxidation protection system disposed on a substrate may comprise a boron-silicon-glass layer formed directly on the composite structure. The boron-silicon-glass layer may comprise a boron compound, a silicon compound, and a glass compound.