Composite Filament for FDM Printing Resolves PLA Brittleness

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Solution Overview

Problem

Polylactic acid (PLA) filaments used in FDM printing exhibit brittleness, poor dimensional stability, and surface defects when fused at temperatures below 210°C, and have inadequate adhesion to printing planes, leading to distortion and incomplete reproduction of intended objects.

Innovation Solution

Filaments comprising a composition of 10-90% polyester, 5-90% polyhydroxyalkanoate, 0-5% cross-linking agent, and 0-50% filler agent, specifically designed to enhance breaking strength, adhesion, and dimensional stability, with a dicarboxylic component comprising aromatic and saturated aliphatic units, and a diol component predominantly from saturated aliphatic diols, are used in the FDM printing process.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If polylactic acid filaments are used in FDM printing, then biodegradability and ease of use are maintained, but breaking strength is insufficient and filaments break during movement

Engineering Contradiction:
Improveease of useVSAvoidbreaking strength
Core Design Contradiction:
Ease of operationVSStrength

Solution Approach 1:

The patent applies composite materials by combining polylactic acid with at least one additional thermoplastic polymer (such as polyethylene terephthalate, polyamide, or polypropylene) to create a composite filament. This composite structure maintains the biodegradability and ease of use of PLA while incorporating the superior strength and flexibility of the additional polymer, thereby preventing filament breakage during FDM printing operations.

Inventive Principle:
Principle #40Composite materials

2Ease of operation

If polylactic acid filaments are used in FDM printing, then biodegradability is maintained, but dimensional stability is poor and distortion occurs after cooling

Engineering Contradiction:
Improveease of useVSAvoiddimensional stability
Core Design Contradiction:
Ease of operationVSStability of the object's composition

Solution Approach 1:

The patent uses composite materials combining PLA with thermoplastic polymers that have better dimensional stability. The additional polymer component compensates for PLA's tendency to distort during cooling, maintaining the intended geometry of printed objects while preserving the biodegradable nature of the composite material.

Inventive Principle:
Principle #40Composite materials

3Use of energy by stationary object

If polylactic acid filaments are fused at temperatures below 210°C, then energy consumption is reduced, but surface defects appear on printed objects

Engineering Contradiction:
Improveenergy consumptionVSAvoidsurface quality
Core Design Contradiction:
Use of energy by stationary objectVSManufacturing precision

Solution Approach 1:

The patent modifies the material composition parameter by incorporating thermoplastic polymers with lower melting points or better flow characteristics. This allows the composite filament to be printed at reduced temperatures (below 210°C) while maintaining adequate surface quality, as the additional polymer enhances melt flow and surface finishing capabilities.

Inventive Principle:
Principle #35Parameter changes

4Ease of operation

If polylactic acid filaments are used in FDM printing, then biodegradability is maintained, but adhesion to printing planes is insufficient and faithful reproduction is not guaranteed

Engineering Contradiction:
Improveease of useVSAvoidreproduction fidelity
Core Design Contradiction:
Ease of operationVSManufacturing precision

Solution Approach 1:

The patent employs composite materials where the additional thermoplastic polymer component provides improved adhesion properties. This enhances the bonding between deposited layers and the printing plane, ensuring faithful reproduction of the three-dimensional model while maintaining the biodegradable characteristic of the composite filament.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The modified filaments demonstrate improved breaking strength and dimensional stability, ensuring faithful reproduction of objects with reduced surface defects and enhanced adhesion to printing surfaces, maintaining biodegradability and ease of use.

Implementation Method 1

0-5% by weight, preferably 0-1% with respect to the sum of components i.-iv., of at least one cross-linking agent and/or chain extender comprising at least one di- and/or multiple functional group compound containing isocyanate, peroxide, carbodiimide, isocyanurate, oxazoline, epoxy, anhydride, or divinylether groups

Methodology Applied
Scientific EffectCross-linking: Chemical Bonding

Implementation Method 2

The filament is thrust by a toothed wheel through a melting unit provided with a nozzle from which the material in the fused state is deposited

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 3

The FDM printing process provides for the deposition of overlapping layers of a filament of thermoplastic material while the latter is in the fused state

Methodology Applied
Scientific EffectCooling and solidification: Freezing

Data Source

PatentEP3319787B1Use of polymer compositions for the production of filaments for fused deposition modelling
Publication Date: 2021.11.17 NOVAMONT SPA
  • EP3319787B1 patent drawingFigure 1
  • EP3319787B1 patent drawing

AI summary

This invention relates to the use of polymer compositions for the production of filaments for use for printing through fused deposition modelling. This invention also relates to the process of printing by fused deposition modelling which uses the said compositions and objects printed which can be obtained by means of the said printing process.