Composite Oxidation Coating for Hydrolytic Stability

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Solution Overview

Problem

Oxidation protection systems for carbon-carbon composite structures face hydrolytic instability due to the water solubility of boron oxide formed at high temperatures, leading to increased oxidation and material loss.

Innovation Solution

A method involving the application of a boron slurry and a silicon slurry, each comprising specific glass compounds and modifiers, is used to form a boron-glass and silicon-glass layer on the composite structure, with cubic boron nitride and colloidal silica enhancing oxidation resistance and water stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If boron carbide and silicon carbide layers are used for oxidation protection, then oxidation resistance is improved, but hydrolytic stability deteriorates due to water solubility of boron oxide

Engineering Contradiction:
Improveoxidation resistanceVSAvoidhydrolytic stability
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent introduces glass compounds (such as borosilicate glass, aluminosilicate glass) as intermediary substances between the boron carbide/silicon carbide layers and the external environment. These glass compounds form a protective glassy matrix that encapsulates the boron oxide, preventing its direct contact with water and eliminating hydrolytic instability while maintaining oxidation protection capabilities.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite oxidation protection system combining boron carbide, silicon carbide, and glass compounds in a multi-phase structure. This composite material integrates the high-temperature oxidation resistance of boron carbide/silicon carbide with the hydrolytic stability and protective properties of glass compounds, achieving both required performance characteristics simultaneously.

Inventive Principle:
Principle #40Composite materials

2Reliability

If boron oxide is formed during high-temperature operation, then oxidation protection function is achieved, but water solubility increases leading to material loss

Engineering Contradiction:
Improveoxidation protection functionVSAvoidcarbon material loss
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The glass compounds act as intermediary substances that trap and stabilize boron oxide within a glassy matrix, preventing its dissolution in water. This intermediary layer maintains the oxidation protection function while eliminating the harmful water solubility of boron oxide, thereby preventing carbon material loss.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent converts the harmful water-soluble boron oxide into a beneficial component by incorporating it within the glass matrix. The boron oxide that would normally cause material loss is transformed into a stable part of the glassy protective layer, turning a detrimental substance into a functional component of the protection system.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively reduces oxidation and improves water stability of the oxidation protection system, maintaining material integrity under high-temperature conditions.

Implementation Method 1

applying a boron slurry and a silicon slurry, each comprising specific glass compounds and modifiers, is used to form a boron-glass and silicon-glass layer on the composite structure

Methodology Applied
Scientific EffectVitrification: Vitrification

Implementation Method 2

The carbon-carbon composite structure is porous and the second pretreating composition penetrates a pore of the composite structure

Methodology Applied
Scientific EffectCapillary action: Capillary Action

Implementation Method 3

heating the carbon-carbon composite structure

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP4279472A1Oxidation protection of composites
Publication Date: 2023.11.22 GOODRICH CORP
  • EP4279472A1 patent drawingFigure 1
  • EP4279472A1 patent drawingFigure 2
  • EP4279472A1 patent drawing

AI summary

Systems and methods for forming an oxidation protection system on a composite structure are provided. In various embodiments, the oxidation protection system comprises a boron-glass layer formed on the composite substrate and a silicon-glass layer formed over the boron-glass layer. Each of the boron-glass layer and the silicon-glass layer include a glass former and a glass modifier. The boron-glass layer includes a boron compound comprising a mixture of boron carbide (B4C) powder and cubic boron nitride (BN) powder.