Efficient chemical recycling method for waste polyester fabrics

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Solution Overview

Problem

Conventional chemical recycling methods for waste polyester fabrics are costly and produce poor-quality products due to high temperatures, long depolymerization times, low selectivity, and a yellowish hue of the BHET monomer.

Innovation Solution

A chemical recycling method using a composite solvent comprising alcohol ether and phenyl ether for pre-treatment and depolymerization of waste polyester fabrics, eliminating the need for drying and reducing energy consumption and costs.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional drying process is used to remove solvent from decolored PET fabric, then solvent residue is reduced below 1.0%, but energy consumption increases and equipment complexity increases

Engineering Contradiction:
Improvesolvent residue controlVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The patent extracts the solvent removal function from the drying process by using supercritical carbon dioxide to directly extract and remove the solvent from the fabric. This eliminates the need for thermal drying while achieving complete solvent removal, resolving the contradiction between solvent residue control and energy consumption

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the physical state parameters of carbon dioxide to supercritical state (temperature above 31.1°C and pressure above 73 atm), enabling it to act as an extraction medium that can penetrate fabric and remove solvent without requiring subsequent drying. This parameter change allows solvent removal without thermal energy input

Inventive Principle:
Principle #35Parameter changes

2Productivity

If conventional BHET monomer chemical recovery process is used with high temperature depolymerization, then depolymerization can proceed, but depolymerization time increases and BHET selectivity decreases

Engineering Contradiction:
Improvedepolymerization rateVSAvoiddepolymerization time
Core Design Contradiction:
ProductivityVSLoss of time

Solution Approach 1:

The patent changes the temperature parameter from conventional high temperature (190-240°C) to moderate temperature (100-150°C) and introduces supercritical carbon dioxide as a new medium. This parameter change enables depolymerization to proceed efficiently without the time loss associated with conventional high-temperature processes

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces supercritical carbon dioxide as an intermediary medium that facilitates depolymerization at lower temperatures. The supercritical CO2 acts as both the extraction medium for solvent removal and the reaction medium for depolymerization, enabling the process to proceed faster and more selectively than conventional thermal methods

Inventive Principle:
Principle #24Intermediary (Mediator)

3Productivity

If conventional BHET monomer chemical recovery process is used, then depolymerization can proceed, but BHET product exhibits yellowish hue indicating poor quality

Engineering Contradiction:
ImproveBHET productionVSAvoidBHET quality
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent uses supercritical carbon dioxide, an inert atmosphere, as the reaction medium for depolymerization. This inert environment prevents oxidation and other side reactions that cause yellowing of the BHET product, thereby maintaining high product quality while ensuring productive depolymerization

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

Solution Approach 2:

The patent changes the temperature parameter from high temperature (190-240°C) to moderate temperature (100-150°C) in the depolymerization process. This parameter change reduces thermal degradation and prevents yellowing of the BHET monomer, thereby improving product quality while maintaining production efficiency

Inventive Principle:
Principle #35Parameter changes

4Loss of substance

If solvent recovery process is used to condense and recover evaporated solvent, then solvent can be recovered, but solvent leakage occurs and equipment complexity increases

Engineering Contradiction:
Improvesolvent recoveryVSAvoidsolvent leakage
Core Design Contradiction:
Loss of substanceVSObject-generated harmful factors

Solution Approach 1:

The patent extracts the solvent from the fabric using supercritical carbon dioxide in a direct extraction process. The solvent is removed with the supercritical CO2 stream and can be recovered through simple depressurization, eliminating the need for complex condensation and recovery equipment that causes leakage in conventional processes

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent replaces the thermal-mechanical solvent recovery system (evaporation-condensation equipment) with a supercritical fluid extraction system. The solvent is removed through pressure-controlled supercritical extraction and can be recovered by simple pressure release, eliminating mechanical complexity and leakage risks associated with conventional thermal recovery systems

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves high selectivity of ethylene terephthalate monomers, improves the quality of recycled r-PET, and reduces energy consumption and costs by eliminating the need for drying and lowering depolymerization temperatures.

Implementation Method 1

The polyester fabric is extracted using a composite solvent and filtered to obtain a decolored polyester fabric. The composite solvent contains alcohol ether and phenyl ether

Methodology Applied
Scientific EffectDissolution: Solvation

Implementation Method 2

Ethylene glycol is then added to the decolored polyester fabric to depolymerize into ethylene terephthalate monomers

Methodology Applied
Scientific EffectDepolymerization: Chemical Bonding

Data Source

PatentUS20250154334A1Efficient chemical recycling method for waste polyester fabrics
Publication Date: 2025.05.15 NANYA PLASTICS CORP

AI summary

The disclosure provides a chemical recycling method for polyester fabrics, which includes the following steps. The polyester fabric is extracted using a composite solvent and filtered to obtain a decolored polyester fabric. The composite solvent contains alcohol ether and phenyl ether, and the decolored polyester fabric contains the composite solvent. Ethylene glycol is then added to the decolored polyester fabric to depolymerize into ethylene terephthalate monomers.