Concentrated Neutral Titanium Dioxide Sol Preparation

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Solution Overview

Problem

Current photoactive, neutral titanium dioxide sols are limited by low titanium dioxide concentration, leading to high solvent content, which complicates their use and transportation due to excessive volume and cost, and restricts their applications.

Innovation Solution

Methods involving washing and dewatering of hydrous titanium dioxide gel with low cation concentration aqueous solvents, followed by peptization with alkaline agents and neutralization with concentrated acids to achieve titanium dioxide sols with concentrations of 30% or greater, maintaining pH neutrality and photocatalytic activity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If photoactive, neutral titanium dioxide sols are prepared with conventional methods, then the sols are stable and neutral in pH, but the titanium dioxide concentration is limited to about 10-15% by weight

Engineering Contradiction:
ImprovepH stabilityVSAvoidtitanium dioxide concentration
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent applies parameter changes by modifying the chemical composition parameters during preparation - specifically using alkaline peptizing agents (like ammonium hydroxide or sodium hydroxide) followed by controlled acid neutralization. This parameter transformation enables the formation of concentrated sols with TiO2 concentrations of 30% or greater while maintaining pH stability in the neutral range of 7-9, resolving the contradiction between concentration and pH stability.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If titanium dioxide sol is prepared with low concentration (10-15%), then the sol is easy to prepare and stable, but it requires substantially large volume of solvent leading to excessive transportation and storage space

Engineering Contradiction:
Improvepreparation easeVSAvoidsolvent volume
Core Design Contradiction:
Ease of manufactureVSVolume of moving object

Solution Approach 1:

The patent applies the extraction principle by removing excess solvent from the system through the peptization and concentration process. By using alkaline peptizing agents to disperse TiO2 particles and then concentrating the sol to 30% or greater TiO2 content, the method extracts unnecessary solvent volume while maintaining sol stability and neutrality, thereby reducing transportation and storage requirements.

Inventive Principle:
Principle #2Taking out (Extraction)

3Object-affected harmful factors

If conventional neutral titanium dioxide sol is used, then the sol is odorless and non-flammable, but the high solvent content (approximately 90% by weight) adds excessive volume and cost

Engineering Contradiction:
Improveodor and flammabilityVSAvoidsolvent content
Core Design Contradiction:
Object-affected harmful factorsVSQuantity of substance

Solution Approach 1:

The patent applies parameter changes by transforming the solvent content parameter from approximately 90% by weight in conventional sols to 70% or less by weight in the concentrated sols. This is achieved through controlled peptization with alkaline agents and subsequent concentration, while maintaining the beneficial properties of being odorless and non-flammable through proper pH control in the neutral range.

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentEP3377446B1Concentrated photoactive, neutral titanium dioxide sol
Publication Date: 2019.04.03 TRONOX LLC
  • EP3377446B1 patent drawingFigure 1
  • EP3377446B1 patent drawingFigure 2
  • EP3377446B1 patent drawingFigure 3

AI summary

The present disclosure relates to methods of preparing sols of titanium dioxide nanoparticles that are photoactive, neutral, and in a substantially concentrated form. The methods particularly provide for concentrated sols in light of washing and dewatering under low cation concentrations and utilizing rapid peptizing through addition of the filter case to the peptizing agent. Concentrated acid may be utilized to maintain high TiO2 concentration while still avoiding precipitation of the colloidal TiO2. Concentrated photoactive, neutral titanium dioxide sols are also provided as well as compositions thereof and photoactive coatings formed therewith.