Conductive Paste Rheology Control for Multilayer Screen Printing

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Solution Overview

Problem

Conductive pastes with high metal powder content face challenges in continuous screen printing on ceramic green sheets, experiencing issues like bleeding, low spots, and shear droop, which hinder the formation of high-definition conductor patterns with thick film thickness and high aspect ratios, especially in mass production scenarios.

Innovation Solution

A conductive paste composition with 70-95 weight % conductive metal powder, a resin, and a solvent, optimized to achieve a specific phase angle range in dynamic viscoelastic measurements, ensuring stable printing properties and preventing defects such as bleeding and shear droop.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If high metal powder content (70-95 wt%) is used in conductive paste, then conductor resistance is reduced and film thickness is increased, but printing defects such as bleeding, low spots, and shear droop occur during continuous screen printing

Engineering Contradiction:
Improveconductor pattern definitionVSAvoidprinting stability
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent applies parameter changes by optimizing the viscosity of the vehicle component within a specific range (10-100 Pa·s at 25°C) and controlling the particle size distribution of metal powder (D50: 1-10 μm, D90: 15-20 μm). These parameter optimizations enable the high metal content paste to maintain stable rheological properties during screen printing, preventing bleeding and shear droop while achieving thick film deposition with high definition patterns.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite materials by formulating a vehicle consisting of multiple resin components (e.g., nitrocellulose, ethyl cellulose, polyvinyl butyral) combined with specific solvents and dispersants. This composite vehicle system provides balanced flow characteristics and adhesion properties, allowing the high metal powder content paste to maintain printing stability and prevent defects during continuous screen printing operations.

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If thick film thickness and high aspect ratio patterns are formed, then conductor resistance is reduced, but continuous printing accuracy deteriorates due to paste defects

Engineering Contradiction:
Improvepattern aspect ratioVSAvoidcontinuous printing capability
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent applies parameter changes by controlling the viscosity of the vehicle within 10-100 Pa·s at 25°C and optimizing metal powder particle size distribution (D50: 1-10 μm, D90: 15-20 μm). These parameters enable the paste to maintain stable flow characteristics during screen printing, allowing continuous printing of high aspect ratio patterns (thickness/width ratio) without bleeding or shear droop defects, thus achieving both thick films and high productivity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies dynamics by formulating the vehicle with resin and solvent components that provide time-dependent rheological behavior. The vehicle maintains higher viscosity at rest to prevent bleeding, but exhibits shear-thinning characteristics during the dynamic screen printing process, allowing smooth paste flow through the screen mesh and squeegee action, thereby enabling continuous high-accuracy printing.

Inventive Principle:
Principle #15Dynamics

3Stability of the object's composition

If solid content of conductive paste is increased to reduce firing shrinkage, then interlayer separation and cracks are minimized, but printing defects such as bleeding and shear droop increase

Engineering Contradiction:
Improvefiring shrinkage consistencyVSAvoidpattern definition
Core Design Contradiction:
Stability of the object's compositionVSManufacturing precision

Solution Approach 1:

The patent applies parameter changes by optimizing the vehicle viscosity to 10-100 Pa·s at 25°C and controlling metal powder particle size (D50: 1-10 μm, D90: 15-20 μm). These parameters enable the high solid content paste (70-95 wt% metal powder) to maintain stable composition during firing with minimal shrinkage, while simultaneously preventing printing defects like bleeding and shear droop through controlled rheological properties.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite materials by formulating a vehicle with multiple resin components (nitrocellulose, ethyl cellulose, polyvinyl butyral) and solvents that provide balanced rheological and adhesive properties. This composite vehicle system allows the high solid content paste to maintain pattern definition during screen printing while ensuring firing shrinkage consistency and preventing interlayer separation or cracks.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables continuous high-accuracy screen printing with reduced defects, allowing for the mass production of multilayer electronic parts with thick film thickness and high aspect ratio patterns, even after 1,000 printing cycles, and ensures excellent via filling properties.

Implementation Method 1

A conductive paste is printed on the green sheet by a screen printing method to form a predetermined conductor pattern

Methodology Applied
Scientific EffectScreen printing:

Implementation Method 2

A conductive paste composition with 70-95 weight % conductive metal powder, a resin, and a solvent, optimized to achieve a specific phase angle range in dynamic viscoelastic measurements, ensuring stable printing properties

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 3

The cut laminated body is fired

Methodology Applied
Scientific EffectSintering: Sintering

Implementation Method 4

the conductive paste is filled in the via hole... Subsequently, the cut laminated body is fired

Methodology Applied
Scientific EffectFiring:

Implementation Method 5

as for the conductive pastes, the followings are used; at least conductive powder, a vehicle including a resin and an organic solvent... the amount of the resin and the solvent to be burnt off during firing is decreased

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentUS7410601B2Conductive paste for multilayer electronic part
Publication Date: 2008.08.12 SHOEI CHEM IND CO LTD

AI summary

Disclosed is a conductive paste for a multilayer electronic part to be screen-printed on a ceramic green sheet, comprising 70-95 weight % of conductive metal powder, a resin, and a solvent, wherein a phase angle δ in a dynamic viscoelastic measurement is within a range of from 43° to 72° at a frequency of 0.05 Hz and is within a range of 63° or less at a frequency of 30 Hz.