COPD Inhaler Formulation Stabilization with HCl

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Solution Overview

Problem

Current pharmaceutical aerosol formulations of glycopyrronium chloride and formoterol are unstable under high temperature and humidity conditions, leading to significant degradation of formoterol and the formation of unwanted degradation products, making them clinically and commercially non-viable.

Innovation Solution

Incorporating an optimized amount of 1M HCl (0.1-0.3 µg/µl) in the formulation, along with removing oxygen from the canister headspace, stabilizes both glycopyrronium chloride and formoterol, ensuring consistent delivery over an extended period.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If pharmaceutical aerosol formulations of glycopyrronium chloride and formoterol are stored under high temperature and humidity conditions, then the formulation remains stable initially, but significant degradation of formoterol occurs and unwanted degradation products form

Engineering Contradiction:
Improveformulation stabilityVSAvoiddegradation of formoterol
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent introduces HCl as an intermediary substance that mediates between the active ingredients and the degrading environment. The HCl maintains an acidic environment that prevents hydrolysis and degradation of formoterol and glycopyrronium chloride, acting as a protective mediator against temperature and humidity-induced degradation

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates an inert chemical environment by establishing acidic conditions with HCl that are chemically resistant to degradation. This inert environment protects the active ingredients from reacting with water or oxygen during storage under high temperature and humidity conditions

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

2Duration of action of stationary object

If the formulation is designed for extended period delivery, then consistent dosing is achieved, but stability under high temperature and humidity deteriorates

Engineering Contradiction:
Improveextended period deliveryVSAvoidstability under high temperature and humidity
Core Design Contradiction:
Duration of action of stationary objectVSReliability

Solution Approach 1:

The patent applies preliminary action by adding HCl to the formulation before storage, which preemptively establishes protective acidic conditions. This preliminary stabilization prevents degradation from occurring during extended storage periods under high temperature and humidity, enabling consistent dosing over time

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent changes the chemical parameter of the formulation by introducing HCl to create an acidic environment. This parameter change from neutral to acidic conditions fundamentally alters the stability characteristics of the formulation, enabling it to maintain reliability during extended storage under harsh conditions

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The stabilization of formoterol and glycopyrronium chloride results in a stable aerosol formulation that maintains effective dosing for an extended period, meeting clinical and commercial viability standards, with reduced levels of degradation products below identification thresholds.

Implementation Method 1

Incorporating an optimized amount of 1M HCl (0.1-0.3 µg/µl) in the formulation, along with removing oxygen from the canister headspace, stabilizes both glycopyrronium chloride and formoterol

Methodology Applied
Scientific EffectChemical stabilization:

Implementation Method 2

pharmaceutical aerosol solution formulations intended for use with pressurized metered dose inhalers

Methodology Applied
Scientific EffectAerosolization: Aerosol

Implementation Method 3

pressurized metered dose inhalers

Methodology Applied
Scientific EffectPressurization: Pressurisation

Data Source

PatentEP2515853B1Combination therapy for COPD
Publication Date: 2014.03.19 CHIESI FARMACEUTICI SPA

AI summary

The invention concerns an aerosol formulation suitable for administering to COPD patients by means of a pressurized metered dose inhaler (pMDI), comprising glycopyrronium chloride in combination with formoterol. The formulation further comprises a HFA propellant, a co-solvent, and an amount of inorganic acid sufficient to stabilize both the glycopyrronium chloride and the formoterol components. Optionally the formulation further comprises beclometasone dipropionate.