Copolyamide Molding Compound Low Water Absorption

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Solution Overview

Problem

Standard polyamides like PA6 and PA66 exhibit high water absorption, leading to dimensional instability and reduced mechanical properties under humid conditions, while partially aromatic polyamides have high melting points and low crystallinity, making them unsuitable for applications requiring dimensional stability and processability.

Innovation Solution

A copolyamide composition comprising 50-95 mol% of a diamine combination of 1,10-decanediamine, 1,11-undecanediamine, or 1,12-dodecanediamine with terephthalic acid, and 5-50 mol% of 2,2,4-trimethylhexamethylenediamine or 2,4,4-trimethylhexamethylenediamine, optimized for melting points between 250°C to 300°C, ensuring high crystallinity and minimal property changes in moist conditions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If standard polyamides (PA6, PA66) are used, then ease of processing is improved, but water absorption increases leading to dimensional instability

Engineering Contradiction:
ImproveprocessabilityVSAvoiddimensional stability
Core Design Contradiction:
Ease of manufactureVSStability of the object's composition

Solution Approach 1:

The invention uses copolyamides containing both aliphatic (PA6, PA66) and aromatic (PA6T, PA6I) units to create a composite material that combines the processability of aliphatic polyamides with the dimensional stability and low water absorption of aromatic polyamides

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention modifies the chemical composition parameters by controlling the ratio of aliphatic to aromatic polyamide units (1:4 to 4:1) to achieve optimal balance between processability and dimensional stability, reducing water absorption to below 2.5%

Inventive Principle:
Principle #35Parameter changes

2Object-affected harmful factors

If partially aromatic polyamides (PA6T/6I) are used, then water absorption is reduced, but melting point increases and crystallinity decreases

Engineering Contradiction:
Improvewater absorptionVSAvoidmelting point
Core Design Contradiction:
Object-affected harmful factorsVSTemperature

Solution Approach 1:

The invention adjusts the ratio of aromatic to aliphatic units and controls crystallization parameters to achieve a melting point range of 180-280°C, optimizing both low water absorption and suitable processing temperature

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates local crystalline regions within the copolyamide structure that provide dimensional stability while maintaining overall processability through controlled crystallinity in specific domains

Inventive Principle:
Principle #3Local quality

3Object-affected harmful factors

If PA10T is used, then water absorption is greatly reduced, but crystallization rate increases causing nozzle freezing

Engineering Contradiction:
Improvewater absorptionVSAvoidcrystallization rate
Core Design Contradiction:
Object-affected harmful factorsVSProductivity

Solution Approach 1:

The invention modifies the copolyamide composition to control crystallization kinetics, achieving a balance where water absorption is reduced while crystallization occurs at manageable rates during injection molding, preventing nozzle freezing

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a dynamic balance between crystallization and melting during the molding process, allowing controlled crystallization in the mold while preventing premature crystallization in the nozzle through composition optimization

Inventive Principle:
Principle #15Dynamics

4Stability of the object's composition

If PA10T is used, then crystallinity is high, but surface quality deteriorates due to nozzle freezing

Engineering Contradiction:
ImprovecrystallinityVSAvoidsurface quality
Core Design Contradiction:
Stability of the object's compositionVSManufacturing precision

Solution Approach 1:

The invention optimizes the copolyamide composition and processing parameters to achieve sufficient crystallinity for dimensional stability while preventing surface defects caused by nozzle freezing through controlled crystallization kinetics

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The copolyamide achieves excellent heat resistance, dimensional stability, and processability with minimal water absorption, maintaining mechanical properties in both fresh and moisture-conditioned states, suitable for applications such as injection molding and fiber composites.

Implementation Method 1

The material is high-melting with a crystallite melting point Tm of 316°C; It is highly crystalline and crystallizes very quickly

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 2

When stored in water, the mechanical properties do not change significantly. The maximum water absorption is relatively high at around 7.5%

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Data Source

PatentEP2451862B1Molding compound on the basis of a copolyamide containing terephthalic acid and trimethylhexamethylene diamine units
Publication Date: 2018.10.03 EVONIK OPERATIONS GMBH
  • EP2451862B1 patent drawingFigure 1

AI summary

A molding compound, containing at least 30% by weight of a copolyamide, which is derived from the following monomers: a) 50 to 95 mole percent of the combination of a diamine, selected from the group consisting of 1,9-nonane diamine, 1,10-decane diamine, 1,11-undecane diamine and 1,12-dodecane diamine, and terephthalic acid, and b) 5 to 50 mole percent of the combination of a diamine, selected from the group consisting of 2,2,4-trimethylhexamethylene diamine, 2,4,4-trimethylhexamethylene diamine, and mixtures thereof, and terephthalic acid, is crystalline and has low water absorption.