Cathode Potential Control in Copper Electrorefining

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Solution Overview

Problem

Current copper electrorefining processes in the industry operate at suboptimal current densities, resulting in lower quality copper products and reduced efficiency due to the formation of nodular and dendritic structures, which decrease the quality and increase production costs.

Innovation Solution

Implementing a potential-controlled electrorefining method where the cathode potential is maintained between -0.30 V to -0.55 V, allowing for higher current densities up to 2000 A/m², and using complex form potential to control the deposition process, thereby preventing dendrite formation and achieving higher purity copper.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If current-controlled electrorefining is used to operate at high current densities, then productivity increases, but the cathode develops nodular and dendritic structures that reduce manufacturing precision and product quality

Engineering Contradiction:
Improvecurrent densityVSAvoidcathode structure quality
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent applies periodic reversal of current direction, changing the operational parameter from unidirectional direct current to alternating current. This parameter change prevents the formation of nodular and dendritic structures on the cathode while maintaining high current densities, thus resolving the contradiction between productivity and manufacturing precision

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent implements periodic reversal of the current direction through the electrolyte. By alternating the current flow direction at regular intervals, the system prevents localized dendrite growth that occurs with continuous unidirectional current, thereby maintaining both high productivity and high manufacturing precision of the cathode structure

Inventive Principle:
Principle #19Periodic action

2Manufacturing precision

If current-controlled electrorefining operates at suboptimal current densities, then manufacturing precision is maintained, but productivity and current efficiency decrease

Engineering Contradiction:
Improvecathode structure qualityVSAvoidproduction rate
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The periodic reversal of current direction enables the system to operate at higher current densities without forming detrimental dendritic structures. The alternating current pattern ensures that no single area accumulates excessive deposits, maintaining manufacturing precision while significantly increasing productivity compared to traditional suboptimal current densities

Inventive Principle:
Principle #19Periodic action

3Ease of operation

If traditional electrorefining processes are used, then operational simplicity is maintained, but production costs increase due to lower efficiency and quality

Engineering Contradiction:
Improveprocess simplicityVSAvoidproduction efficiency
Core Design Contradiction:
Ease of operationVSProductivity

Solution Approach 1:

The periodic current reversal mechanism is integrated into the existing electrorefining setup, requiring minimal additional equipment. The process maintains ease of operation by using standard power supply equipment capable of alternating current output, while dramatically improving production efficiency and current efficiency through the periodic action principle

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in copper with a purity greater than 99.95%, faster production, and increased current efficiency, reducing production costs and improving the quality of the copper product.

Implementation Method 1

an anode made of impure copper obtained during a fire refining process or from other sources such as recycling, scrap etc. is subjected to electrorefining. During an anodic process, copper is dissolved and aqueous solution is obtained according to the following basic reaction: anode: Cu → Cu²⁺ + 2e⁻

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Implementation Method 2

A sheet of pure copper or acid-resistant steel (stainless steel) provides the cathode on which metallic copper is deposited according to the following basic reaction: cathode: Cu²⁺ + 2e⁻ → Cu

Methodology Applied
Scientific EffectElectrodeposition: Electrodeposition

Data Source

PatentEP2783026B1A method for industrial copper electrorefining
Publication Date: 2023.06.07 NANOMETALLURGY
  • EP2783026B1 patent drawingFigure 1
  • EP2783026B1 patent drawingFigure 2
  • EP2783026B1 patent drawingFigure 3a~3d

AI summary

A method of copper electrorefining is disclosed. The method includes arranging at least one anode of copper material to be refined in contact with an electrolyte solution and arranging at least one cathode in contact with the electrolyte solution. The anode and cathode are connected electrically to an electrical source, and the source is operated under potential controlled conditions. The electrical potential at the cathode is -0.30 V to -0.55 V with respect to the copper material at the anode, thereby causing the deposition of electrorefined copper at the cathode. The method also includes potentiostatic pulse electrolysis (PPE) and periodic potential reversal (PPR) in order to produce a copper deposit having a controllable structure, for example in terms of roughness or porosity. An apparatus for performing potential controlled electrolysis is also disclosed.