Copper Hydroxide Bicarbonate Complexes for Fungicidal Ion Release

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing crop protection agents with copper-based fungicides face limitations in achieving high availability of free copper ions, which is crucial for effective fungicidal activity, often requiring acidification to enhance ion availability.

Innovation Solution

A combination of copper hydroxide with potassium or sodium bicarbonate, forming aquo-carbonato complexes that increase the solubility and release of free, fungicidally active copper ions, utilizing docusate sodium and sodium dodecyl sulfate as wetting agents to enhance the synergistic effect.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If copper hydroxide is used as a fungicidal agent, then fungicidal activity is provided, but availability of free copper ions is insufficient

Engineering Contradiction:
Improvefungicidal activityVSAvoidavailability of free copper ions
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

Bicarbonate ions serve as an intermediary that facilitates the release of copper ions from copper hydroxide through complex formation. The bicarbonate forms aquo-carbonatato complexes with copper, which increases the solubility product and enables greater release of free copper ions without requiring acidification.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention changes the chemical parameters of the spray solution by introducing bicarbonate ions, which alter the equilibrium conditions for copper ion release. This parameter change (addition of bicarbonate) shifts the solubility equilibrium to favor greater copper ion availability while maintaining a neutral to slightly alkaline pH.

Inventive Principle:
Principle #35Parameter changes

2Quantity of substance

If acidification is applied to enhance copper ion availability, then free copper ion availability increases, but plant safety is compromised due to phytotoxic effects

Engineering Contradiction:
Improveavailability of free copper ionsVSAvoidphytotoxic effects
Core Design Contradiction:
Quantity of substanceVSObject-affected harmful factors

Solution Approach 1:

Instead of changing pH through acidification, the invention changes the chemical environment by adding bicarbonate ions. This alternative parameter change achieves increased copper ion availability through complex formation while maintaining pH levels that prevent phytotoxicity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

Bicarbonate acts as a mediator that enables copper ion release without the need for acidification. The bicarbonate-copper complexes serve as an intermediate pathway that decouples copper ion availability from pH reduction, thereby avoiding phytotoxic effects.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Quantity of substance

If copper salt solubility is increased, then fungicidal efficacy is improved, but control over copper ion release becomes difficult

Engineering Contradiction:
Improvecopper ion releaseVSAvoidcontrol over phytotoxicity
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

Bicarbonate ions serve as a controllable intermediary that regulates copper ion release through reversible complex formation. The equilibrium between bicarbonate-copper complexes and free copper ions can be controlled by adjusting bicarbonate concentration, providing a buffer system that maintains copper availability while preventing excessive release that would cause phytotoxicity.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This combination significantly improves fungicidal efficacy while maintaining plant safety by optimizing copper ion availability and solubility, preventing phytotoxic effects, and demonstrating a clear synergistic effect in various copper formulations.

Implementation Method 1

the formation of intermediate carbonato-copper complexes with a hydrogen carbonate before it is fixed as basic copper carbonate

Methodology Applied
Scientific EffectComplex formation: Chemical Bonding

Implementation Method 2

the presence of dissolved bicarbonate ions and the associated formation of the aforementioned complex structures leads to an increase in the solubility product of the copper component used, and thus to an increased release of free, fungicidal Cu-ions

Methodology Applied
Scientific EffectSolubility product increase: Solvation

Implementation Method 3

the effectiveness can be improved by adding at least one wetting agent. Sodium dodecyl sulfate and/or docusate sodium, for example, can be used as wetting agents

Methodology Applied
Scientific EffectWetting: Wetting

Data Source

PatentEP3503731B1Copper-containing preparation for use as a plant protection agent
Publication Date: 2021.03.03 CERTIS EURO BV
  • EP3503731B1 patent drawingFigure 1
  • EP3503731B1 patent drawingFigure 2
  • EP3503731B1 patent drawingFigure 3

AI summary

The invention relates to a preparation for use as a plant protection agent, wherein at least one copper-containing component and at least one alkaline and/or bicarbonate-ion liberating component is contained. The preparation can be used in particular as a fungicide and also preferably as a liquid preparation based on water or as a tank mixture or as a ready-to-use preparation, preferably in the form of powder or granules.