Core-Shell Nanoprecipitated Calcium Carbonate for Whiteness and Cost

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Solution Overview

Problem

Low-grade limestone with high impurity content is often discarded or used at low value due to its impact on the whiteness of nanoprecipitated calcium carbonate, as existing methods for improving whiteness, such as lime sorting and chemical whitening, are labor-intensive or alter the pH of calcium carbonate, limiting their effectiveness.

Innovation Solution

A method for producing nanoprecipitated calcium carbonate with a core-shell structure by using low-grade limestone as the core and high-grade limestone as the shell, where the core is coated with a high-whiteness precipitated calcium carbonate layer through calcination, slaking, and controlled carbonation processes, ensuring uniform shell formation and morphology.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If low-grade limestone with high impurity content is used to produce nanoprecipitated calcium carbonate, then production cost is reduced, but the whiteness of the product deteriorates due to impurities such as iron and manganese

Engineering Contradiction:
Improveproduction costVSAvoidwhiteness
Core Design Contradiction:
Ease of manufactureVSIllumination intensity

Solution Approach 1:

The patent divides the calcium carbonate particles into core and shell structures, where the core is formed from low-grade limestone (providing cost advantage) and the shell is formed from high-purity calcium carbonate (providing whiteness). This segmentation allows each part to fulfill its specific function independently, resolving the contradiction between cost and whiteness.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent creates a composite nanoprecipitated calcium carbonate material with core-shell structure, combining low-grade limestone core with high-purity calcium carbonate shell. This composite structure integrates the cost benefits of low-grade limestone with the aesthetic benefits of high-purity material, simultaneously achieving both low production cost and high whiteness.

Inventive Principle:
Principle #40Composite materials

2Illumination intensity

If chemical whitening methods are used to remove impurities, then the whiteness of the product is improved, but the pH of calcium carbonate is altered, affecting its basic properties

Engineering Contradiction:
ImprovewhitenessVSAvoidpH
Core Design Contradiction:
Illumination intensityVSStability of the object's composition

Solution Approach 1:

The patent segments the whitening function from the bulk calcium carbonate material by creating a shell layer that provides whiteness without altering the pH of the core calcium carbonate. The shell acts as a protective layer that prevents impurity exposure while maintaining the chemical stability of the core.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The high-purity calcium carbonate shell acts as an intermediary layer between the impure core and the external environment. This shell mediates the interaction between impurities and the bulk material, providing whiteness while preserving the original pH and chemical properties of the calcium carbonate.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Illumination intensity

If lime sorting methods are used to separate high-quality lime, then the whiteness of the product is improved, but the process becomes labor-intensive and automated sorting cannot be performed

Engineering Contradiction:
ImprovewhitenessVSAvoidautomation
Core Design Contradiction:
Illumination intensityVSEase of operation

Solution Approach 1:

The patent employs self-service principles by allowing the calcium carbonate particles to self-assemble into core-shell structures during the carbonation process. The system automatically separates and organizes particles based on their properties without requiring external manual sorting operations, enabling automated production while maintaining high whiteness.

Inventive Principle:
Principle #25Self-service

Solution Approach 2:

The patent replaces mechanical sorting systems with a chemical process-based separation mechanism. Instead of using physical sorting equipment, the invention uses differential carbonation rates and particle formation mechanisms to automatically separate high-purity core particles from impure outer layers, enabling automated operation.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method improves the whiteness of nanoprecipitated calcium carbonate while reducing production costs and ensuring consistent morphology, enhancing its application in fields like soft PVC, where high whiteness is critical.

Implementation Method 1

calcining low-grade limestone to obtain quick lime

Methodology Applied
Scientific EffectCalcination: Thermolysis

Implementation Method 2

slaking the quick lime and removing slag to obtain a first lime slurry

Methodology Applied
Scientific EffectSlaking: Hydrolysis

Implementation Method 3

carbonation of core-nanoprecipitated calcium carbonate: feeding the first lime slurry into a carbonation tower for carbonation reaction

Methodology Applied
Scientific EffectCarbonation: Precipitation

Data Source

PatentEP3738926B1Preparation method for nanoprecipitated calcium carbonate having core-shell structure
Publication Date: 2023.07.19 GUANGXI HUANA NEW MATERIALS TECH CO LTD
  • EP3738926B1 patent drawingFigure 1

AI summary

A preparation method for nanoprecipitated calcium carbonate having a core-shell structure, comprising the following steps: (1) the preparation of core-nanoprecipitated calcium carbonate: calcining low-grade limestone to obtain quicklime, digesting and removing slag, and adjusting the solid content of a first lime slurry; delivering the first lime slurry into a carbonation tower for a carbonation reaction to obtain a core-nanoprecipitated calcium carbonate suspension; (2) the coating of the shell: calcining high-grade limestone to obtain quicklime, digesting and removing slag, and adjusting the solid content of a second lime slurry; to coat a shell, mixing the core-nanoprecipitated calcium carbonate suspension with 10-30 wt.% of the second lime slurry, and preparing a suspension of nanoprecipitated calcium carbonate having a core-shell structure by employing a method of carbonation or a method of aging, obtaining nanoprecipitated calcium carbonate having a core-shell structure after post-treatment. The preparation method controls the shell coating process, and ensures that the nanoprecipitated calcium carbonate having a core-shell structure has a cube-like shape.