Core-shell polymer particles for paper sizing

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Solution Overview

Problem

Current surface sizing systems for cellulosic products, such as paper, face challenges in achieving optimal water resistance and efficiency, as measured by the Cobb method, and often require expensive monomers.

Innovation Solution

The development of core-shell polymer particles with a specific monomer composition, where the core and shell are polymerized from a combination of branched alkyl (meth)acrylates, styrene, and acrylonitrile, with a high percentage of branched C3-10 alkyl (meth)acrylate in the shell, providing improved sizing performance and allowing for the replacement of expensive monomers without compromising efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If traditional surface sizing systems are used, then water resistance is achieved, but expensive monomers are required and sizing efficiency can be improved

Engineering Contradiction:
Improvesizing efficiencyVSAvoidcost of monomers
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The invention uses composite polymer particles with a core-shell structure where the core contains hydrophobic branched alkyl (meth)acrylate monomers for water resistance and the shell contains styrene and acrylonitrile for durability and adhesion. This composite structure achieves superior sizing efficiency while reducing dependence on expensive traditional sizing monomers.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The core-shell structure distributes different functional properties to different regions: the core provides hydrophobicity for water resistance, while the shell provides mechanical durability and adhesion. This local differentiation of properties optimizes sizing performance across different functional requirements.

Inventive Principle:
Principle #3Local quality

2Object-affected harmful factors

If high percentage of branched alkyl (meth)acrylate is used, then water resistance is improved, but cost increases

Engineering Contradiction:
Improvewater absorptivenessVSAvoidcost of branched alkyl (meth)acrylate
Core Design Contradiction:
Object-affected harmful factorsVSQuantity of substance

Solution Approach 1:

The invention optimizes the ratio of branched alkyl (meth)acrylate to other monomers (styrene and acrylonitrile) to achieve the minimum effective concentration for water resistance while reducing overall cost. The core-shell structure concentrates the hydrophobic monomers where most needed, allowing parameter optimization.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention replaces portions of expensive branched alkyl (meth)acrylate monomers with more cost-effective styrene and acrylonitrile in the shell structure, maintaining water resistance performance while reducing material costs.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Reliability

If core-shell structure is used, then sizing efficiency is enhanced, but manufacturing complexity increases

Engineering Contradiction:
Improvesizing efficiencyVSAvoidpolymerization process complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The core-shell structure is formed through sequential polymerization where the core is formed first, followed by deposition of the shell material. This preliminary formation of the core structure simplifies the overall process compared to simultaneous formation of complex multifunctional particles.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The core-shell polymer particles demonstrate enhanced sizing efficiency, reducing water absorptiveness of paper and maintaining performance even when reducing the ratio of branched alkyl (meth)acrylate, while also being cost-effective by using a styrene-free or reduced styrene formulation.

Implementation Method 1

the core polymer and the shell polymer of the core/shell polymer particle are polymerized from monomers comprising at least 40%, preferably at least 50%, by weight of monomers selected from branched C 3-10 -alkyl (meth)acrylate

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Implementation Method 2

polymer particles having a core-shell structuring with a specific formulation have a sizing efficiency better than polymer particles containing the same monomers in a random polymer structure

Methodology Applied
Scientific EffectHydrophobic effect: Hydrophobe

Data Source

PatentEP3344699B1Core/shell polymer particles as surface sizing agents
Publication Date: 2022.01.12 KEMIRA OY
  • EP3344699B1 patent drawingFigure 1
  • EP3344699B1 patent drawingFigure 2

AI summary

The present invention provides a core/shell polymer particle for surface sizing of cellulosic products, wherein the core polymer and the shell polymer of the core/shell polymer par- ticle are polymerized from monomers comprising at least 40%, by weight of monomers selected from branched C3-10- alkyl (meth)acrylate, styrene, linear C1-10-alkyl (meth)acry- late, and acrylonitrile, based on the total weight of the mon- omers of the core/shell polymer particle; provided that the polymer of the core/shell polymer particle comprises at least 40% by weight of branched C3-6-alkyl (meth)acrylate and at least 50% by combined weight of branched C3-10- alkyl (meth)acrylate and styrene, linear C1-10-alkyl (meth)acrylate, and/or acrylonitrile, based on the total weight of the monomers of the core/shell polymer particle.