Core-Shell Toner with Borax Coupling Agent

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Solution Overview

Problem

Chemically prepared toners face challenges in achieving low-temperature fusing while maintaining stability during shipping and storage, as existing formulations often require trade-offs between fusing properties and storage robustness, and most plasticizing agents migrate to the toner surface, affecting print quality and storage stability.

Innovation Solution

A chemically prepared toner composition with a core-shell structure, where a crystalline polyester resin acts as a plasticizing agent within the core and an amorphous polyester resin forms the shell, both with specific glass transition and melt temperatures, and a borax coupling agent is added to the surface to enhance adhesion and stability, allowing for low-temperature fusing and improved storage properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Temperature

If a styrene-acrylic copolymer latex binder is used to achieve low-temperature fusing, then the fuse window low end is reduced, but the toner becomes vulnerable to caking or blocking during shipping and storage

Engineering Contradiction:
Improvefuse window low endVSAvoidship/storage stability
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

The invention uses a composite binder system comprising both styrene-acrylic copolymer (providing low-temperature fusing) and polyester resin (providing ship/storage stability). This composite approach allows the toner to achieve low end of fuse window of 165°C or lower while simultaneously passing ship/storage tests without caking or blocking.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention applies different functional properties to different components of the binder system: the styrene-acrylic copolymer is optimized for fusing performance (low glass transition temperature) while the polyester resin is optimized for mechanical strength and storage stability. Each component performs its specialized function locally within the composite binder system.

Inventive Principle:
Principle #3Local quality

2Temperature

If most plasticizing agents are used to reduce fusing temperature, then low-temperature fusing is achieved, but the plasticizing agents migrate to the toner surface affecting print quality and storage stability

Engineering Contradiction:
Improvefusing temperatureVSAvoidprint quality
Core Design Contradiction:
TemperatureVSManufacturing precision

Solution Approach 1:

The polyester resin acts as an intermediary substance that provides plasticizing effects (reducing fusing temperature) without the migration problem. It mediates between the need for low fusing temperature and the need to maintain surface quality by remaining stable and non-migrating while still enabling low-temperature fusion.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention changes the chemical parameters of the plasticizing agent by selecting polyester resin with specific properties (glass transition temperature of 55°C or higher) that prevent surface migration while maintaining the ability to facilitate low-temperature fusing through controlled melting behavior.

Inventive Principle:
Principle #35Parameter changes

3Strength

If polyester binder resins are used to improve mechanical properties and pigment compatibility, then durability and color gamut are enhanced, but the polymerization cycle time increases and molecular weight is limited

Engineering Contradiction:
Improvemechanical propertiesVSAvoidpolymerization cycle time
Core Design Contradiction:
StrengthVSLoss of time

Solution Approach 1:

The invention segments the binder system into multiple components (styrene-acrylic copolymer and polyester resin) that can be separately optimized and combined. This allows the polyester resin to provide mechanical strength and pigment compatibility without requiring lengthy polymerization cycles, as the resin can be pre-synthesized and then incorporated into the toner formulation.

Inventive Principle:
Principle #1Segmentation

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The toner achieves low-temperature fusing with enhanced stability during shipping and storage, reducing fine particle formation and maintaining print quality by controlling the crystalline polyester resin's melting point and using borax to prevent surface migration and improve pH resistance.

Implementation Method 1

enabling the formation of hydrogen bonds between polymer chains which assists in the anchoring or binding of the third polymer found in the shell onto the outer surface of the toner core

Methodology Applied
Scientific EffectHydrogen bonding:

Implementation Method 2

The melting point of the crystalline polyester is preferred in the range from 70° C. to 100° C., more preferably about 80° C. to fuse at low temperatures

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 3

an amorphous polyester resin having a high glass transition temperature of at least 55° C.

Methodology Applied
Scientific EffectGlass transition:

Data Source

PatentUS9671709B2Chemically prepared core shell toner formulation including a borax coupling agent and a plasticizing agent in the core
Publication Date: 2017.06.06 LEXMARK INTERNATIONAL INC

AI summary

A chemically prepared toner composition according to one example embodiment includes a core including a first polymer binder, a second polymer binder, a colorant and a release agent; a shell that is formed around the core and includes a third polymer binder; and a borax coupling agent between the core and the shell. The first and third polymer binders are different amorphous polyester resins. The second polymer binder is a crystalline polyester resin and acts as a plasticizing agent in the core. The borax coupling agent assists in adhering the shell to the outer surface of the core. Optionally, the toner of the present invention may be finished with a set of extra particulate additives.