Conductive Hybrid Material for Fuel Cell Catalysts

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Solution Overview

Problem

Existing catalysts for hydrogen oxidation and generation reactions, such as nickel compounds and platinum group elements, face challenges with high overvoltage and cost, and covalent organic frameworks lack electron conductivity, making them inefficient for use in electrode materials and catalysts involving electron transfer reactions.

Innovation Solution

An electrically conductive hybrid material is developed by coordinating platinum group elements with a covalent organic framework, which includes triazine rings and a conductor material like carbon, enhancing catalytic activity and conductivity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If platinum group elements are used as catalysts for hydrogen oxidation and generation reactions, then catalytic activity is improved, but cost increases

Engineering Contradiction:
Improvecatalytic activityVSAvoidcost
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent replaces expensive platinum group element catalysts with non-noble metal catalysts (such as iron, nickel, cobalt, or their oxides, hydroxides, or sulfides) that are significantly cheaper while maintaining adequate catalytic activity for hydrogen oxidation and generation reactions in fuel cells and electrolyzers

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent employs composite catalyst structures combining non-noble metals with support materials (such as carbon materials, metal oxides, or conductive polymers) to enhance the catalytic activity and stability of the inexpensive non-noble metal catalysts, making them viable alternatives to platinum group elements

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If nickel compounds are used as hydrogen generation catalysts, then cost is reduced, but hydrogen generation overvoltage increases by 100 mV or more compared to platinum

Engineering Contradiction:
ImprovecostVSAvoidenergy consumption
Core Design Contradiction:
Quantity of substanceVSUse of energy by moving object

Solution Approach 1:

The patent modifies the physical and chemical parameters of non-noble metal catalysts through controlled synthesis conditions, particle size control, phase composition adjustment, and surface treatment to optimize their catalytic properties and reduce overvoltage, thereby lowering energy consumption while maintaining cost advantages

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates composite structures where non-noble metals are combined with conductive materials or other metal compounds to enhance electron transfer efficiency and reduce polarization resistance, effectively lowering the hydrogen generation overvoltage and energy consumption

Inventive Principle:
Principle #40Composite materials

3Stability of the object's composition

If covalent organic framework is used as catalyst support, then durability is improved, but electron conductivity is insufficient for electrode catalyst applications

Engineering Contradiction:
ImprovedurabilityVSAvoidelectron conductivity
Core Design Contradiction:
Stability of the object's compositionVSReliability

Solution Approach 1:

The patent develops composite materials combining covalent organic frameworks with conductive materials (such as graphene, carbon nanotubes, conductive polymers, or metal nanoparticles) to create a hybrid structure that inherits the high durability and porosity of COFs while gaining the electron conductivity needed for electrocatalytic applications

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent introduces conductive components specifically at the active catalytic sites or interfaces of the COF structure, maintaining the bulk COF's stability and porosity while creating localized conductive pathways that enable efficient electron transfer where needed for electrocatalysis

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The hybrid material achieves improved catalytic activity with reduced metal loading, lower energy consumption, and increased electron transfer efficiency, making it suitable for hydrogen oxidation, generation, and oxygen reduction reactions.

Implementation Method 1

The covalent organic framework is a porous crystalline polymer having meso- or micro-sized pores

Methodology Applied
Scientific EffectPorous structure: Porosity

Implementation Method 2

an electrically conductive hybrid material including a covalent organic framework

Methodology Applied
Scientific EffectElectrical conduction: Conduction (electrical)

Data Source

PatentEP3190157B1Conductive hybrid material including covalent organic structure
Publication Date: 2019.08.07 PANASONIC HOLDINGS CORP
  • EP3190157B1 patent drawingFigure 1(a)~2(b)
  • EP3190157B1 patent drawingFigure 3~5(b)
  • EP3190157B1 patent drawingFigure 6~7

AI summary

An electrically conductive hybrid material includes: a covalent organic framework having pores; and a conductor material, wherein the covalent organic framework is supported on the conductor material. The covalent organic framework that does not have electron conductivity is supported on the conductor material such as a carbon material, thereby can be given the electron conductivity, and becomes usable as such a catalyst material and such an electrode material, which involve the electron transfer, these materials including an electrode catalyst material of a fuel cell, and the like.