Cross-linked Polycarbonate Flame Retardance

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Solution Overview

Problem

Conventional polycarbonate compositions fail to achieve UL 94 V0 and 5VA performance characteristics, especially in thin-walled applications, due to poor flame retardance and drippage issues, while maintaining necessary physical and mechanical properties.

Innovation Solution

A cross-linked polycarbonate composition derived from non-cross-linked polycarbonates with 0.5 mol% to 5 mol% endcap groups from monohydroxybenzophenone and a flame retardant, such as potassium perfluorobutane sulfonate, which achieves UL94 5VA rating at thicknesses of 1.5 mm or less without impact modifiers, brominated, or chlorinated flame retardants.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional polycarbonate compositions are used, then transparency and mechanical properties are maintained, but flame retardance and drippage resistance are insufficient especially in thin-walled applications

Engineering Contradiction:
Improveflame retardanceVSAvoiddrippage
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters by incorporating specific flame retardant compounds (potassium perfluorobutane sulfonate and potassium diphenyl sulfone-3-sulfonate) at optimized concentrations (0.06-0.10 wt% and 0.08-0.12 wt% respectively) to achieve UL 94 V0 and 5VA ratings while maintaining transparency and mechanical properties in thin-walled applications

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system by combining polycarbonate resin with multiple flame retardant additives and processing aids, forming a multi-component composition that achieves synergistic flame retardance without compromising the base polymer's transparency and mechanical performance

Inventive Principle:
Principle #40Composite materials

2Reliability

If flame retardants are added to improve flame resistance, then UL 94 V0 and 5VA ratings are achieved, but transparency and mechanical properties may deteriorate

Engineering Contradiction:
Improveflame retardanceVSAvoidmechanical properties
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent optimizes the concentration parameters of flame retardants to extremely low levels (0.06-0.10 wt% for potassium perfluorobutane sulfonate, 0.08-0.12 wt% for potassium diphenyl sulfone-3-sulfonate) to achieve UL 94 V0 and 5VA ratings while minimizing impact on transparency and mechanical properties

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces processing aids as intermediary substances to facilitate the uniform dispersion of flame retardants at low concentrations, ensuring effective flame retardance while maintaining the mechanical integrity and transparency of the polycarbonate matrix

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If brominated or chlorinated flame retardants are used, then flame resistance is improved, but environmental and safety concerns increase

Engineering Contradiction:
Improveflame retardanceVSAvoidenvironmental impact
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent replaces harmful brominated and chlorinated flame retardants with environmentally benign alternatives (potassium perfluorobutane sulfonate and potassium diphenyl sulfone-3-sulfonate) that provide equivalent or superior flame retardance (UL 94 V0 and 5VA ratings) without the toxic byproducts and environmental persistence associated with traditional halogenated additives

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition exhibits improved flame retardance, transparency, and mechanical properties, including impact strength and ductility, while maintaining chemical resistance and weatherability, suitable for thin-walled articles.

Implementation Method 1

a cross-linked polycarbonate, the cross-linked polycarbonate derived from a non-cross-linked polycarbonate comprising 0.5 mol% to 5 mol% endcap groups that are derived from a monohydroxybenzophenone

Methodology Applied
Scientific EffectPhotopolymerisation: Photopolymerisation

Data Source

PatentEP2935400B1Cross-linked polycarbonate resin with improved chemical and flame resistance
Publication Date: 2018.05.30 SABIC GLOBAL TECHNOLOGIES BV
  • EP2935400B1 patent drawingFigure 1~2
  • EP2935400B1 patent drawingFigure 3
  • EP2935400B1 patent drawingFigure 4~5

AI summary

Disclosed herein are compositions including a cross-linked polycarbonate. The cross-linked polycarbonate may be derived from a polycarbonate having about 0.5 mol% to about 5 mol% endcap groups derived from a monohydroxybenzophenone. A plaque including the composition can achieve a UL94 5VA rating. Also disclosed herein are articles including the compositions, methods of using the compositions, and processes for preparing the compositions.