Crumbly MGDA-Na3 Phase for High-Yield Crystallization

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Solution Overview

Problem

Current processes for preparing solid crystalline MGDA-Na3 are inefficient, leading to low yield, high energy consumption, equipment space requirements, contamination, and significant waste streams, with challenges in achieving high crystallinity and maintaining free-flowing properties, especially under humid conditions.

Innovation Solution

A crumbly phase composition with 70-87 wt% MGDA-Na3 and 13-30 wt% water is developed, which is dried to produce high-quality, high-crystallinity MGDA-Na3 with predominantly crystal type I, avoiding pasty phases and reducing water circulation, thereby improving handling and reducing waste.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If MGDA-Na3 is prepared as an amorphous solid, then the preparation process is simple, but the material becomes hygroscopic and loses free-flowing properties under humid conditions

Engineering Contradiction:
Improvepreparation simplicityVSAvoidfree-flowing properties under humidity
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent changes the physical state parameter of MGDA-Na3 from amorphous to crystalline form. This parameter change fundamentally alters the material's properties, making it less hygroscopic and maintaining free-flowing characteristics even under humid storage conditions, while still allowing for relatively simple preparation processes.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes phase transition from amorphous solid to crystalline solid. By controlling the crystallization process, the patent achieves a stable crystalline phase that resists moisture absorption and maintains flowability, resolving the contradiction between ease of preparation and reliability under humidity.

Inventive Principle:
Principle #36Phase transitions

2Reliability

If conventional processes are used to prepare crystalline MGDA-Na3, then some crystalline form is obtained, but the yield is low and energy consumption is high

Engineering Contradiction:
Improvecrystalline form qualityVSAvoidyield and energy efficiency
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent employs preliminary action by adding seed crystals before the crystallization process. This pre-seeding approach guides the crystallization to proceed efficiently toward the desired crystal type, improving both yield and energy efficiency by avoiding the need for extensive process optimization and reducing energy-intensive trial-and-error adjustments.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention optimizes key process parameters including temperature, concentration, and pH to achieve high-yield crystallization with lower energy consumption. By carefully controlling these parameters, the patent achieves high productivity while maintaining reliable crystalline form quality.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If conventional crystallization processes are used, then crystalline MGDA-Na3 is obtained, but significant waste streams are generated

Engineering Contradiction:
Improvecrystalline product qualityVSAvoidwaste stream generation
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The patent applies discarding and recovering by implementing a mother liquor recycling step. The mother liquor containing dissolved MGDA-Na3 and other components is recovered and fed back into the crystallization process, significantly reducing waste stream generation while maintaining consistent crystalline product quality through controlled crystallization conditions.

Inventive Principle:
Principle #34Discarding and recovering

4Productivity

If equipment for spray granulation is used, then solid MGDA-Na3 can be produced, but the equipment space requirement is large

Engineering Contradiction:
Improvesolid product productionVSAvoidequipment space
Core Design Contradiction:
ProductivityVSArea of stationary object

Solution Approach 1:

The patent replaces complex mechanical spray granulation equipment with a simpler crystallization-based process. By using controlled crystallization in a less space-intensive setup, the invention achieves solid MGDA-Na3 production with reduced equipment space requirements while maintaining productivity through efficient crystallization kinetics and seed crystal technology.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves high yield and quality of crystalline MGDA-Na3 with improved free-flowing properties and reduced waste, maintaining crystallinity and free-flowing characteristics at high humidity, and produces spheroidal particles suitable for detergent applications.

Implementation Method 1

a process wherein this crumbly phase composition is dried to give crystalline MGDA-Na3 product

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 2

Some varieties of crystalline MGDA-Na3 (the trisodium salt of methyl glycine-N,N-diacetic acid) are known in the art, recognizable via XRD-analysis, yielding different characteristic diffraction patterns

Methodology Applied
Scientific EffectCrystallisation: Crystallisation

Data Source

PatentUS12258541B2Crumbly phase composition of methylglycine N,N diacetic acid
Publication Date: 2025.03.25 AKZO NOBEL CHEMICALS INTERNATIONAL BV

AI summary

The present invention relates to a crumbly phase composition containing on total weight of the composition(i) 70-87 wt % of organic compounds and salts thereof containing 85 to 100 wt % on total organic compounds and salts thereof of MGDA-Na3, wherein at least 60 wt % of the MGDA-Na3 is crystalline, and(ii) 13-30 wt % of waterThe invention furthermore relates to a process to prepare the above composition and a process to prepare crystals of MGDA-Na3 by drying the above composition.