Cryogenic Methane Separation With Nitrogen Flammability Control

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Solution Overview

Problem

Cryogenic distillation for methane purification from biogas faces the challenge of flammability risks due to oxygen accumulation in the distillation column, which existing methods fail to adequately address, particularly in ensuring operation outside the flammability zone.

Innovation Solution

Incorporating a nitrogen-rich flow into the distillation column, specifically at the bottom, to enrich nitrogen composition and avoid the flammability zone, thereby preventing oxygen accumulation and ensuring safe operation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If cryogenic distillation is used for methane purification, then high purification yield is achieved, but oxygen accumulation creates flammability risks

Engineering Contradiction:
Improvepurification yieldVSAvoidflammability risk
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

A nitrogen-rich stream is introduced as an intermediary substance into the distillation column to prevent oxygen accumulation. The nitrogen acts as a buffer gas that displaces oxygen from the flammability zone, allowing the distillation process to continue at high efficiency without creating explosive conditions.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates an inert atmosphere within the distillation column by introducing nitrogen-rich gas. This inert environment prevents the formation of flammable mixtures between methane and oxygen, allowing the cryogenic distillation process to operate safely while maintaining high purification yields.

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

2Reliability

If nitrogen-rich flow is added to prevent flammability, then safety is improved, but process complexity increases

Engineering Contradiction:
Improveoperational safetyVSAvoidprocess complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The nitrogen-rich stream serves multiple functions simultaneously: it prevents oxygen accumulation in the flammability zone, maintains proper column pressure, and facilitates continuous operation. This multi-functionality reduces the need for additional separate safety systems, thereby limiting the increase in process complexity.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

The patent modifies the compositional parameters of the feed stream by adding nitrogen-rich gas, changing the overall gas composition to remain outside the flammability zone. This parameter change approach is simpler than installing complex safety monitoring and control systems.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively prevents flammability issues by maintaining the distillation column operation outside the flammability zone, ensuring safe and efficient methane purification while maintaining high yields and minimizing maintenance.

Implementation Method 1

Another solution for the separation is cryogenic distillation as described in WO-A-09/004207

Methodology Applied
Scientific EffectCryogenic distillation: Distillation

Implementation Method 2

the feed stream is sent to a condenser-reboiler where it partially vaporizes the bottom liquid to form a vaporized gas, the fully or partially liquefied feed stream is sent from the condenser-reboiler to the column

Methodology Applied
Scientific EffectPhase change: Phase Change

Implementation Method 3

the vaporized gas is mixed with nitrogen-rich flow

Methodology Applied
Scientific EffectGas mixing:

Implementation Method 4

the feed stream is sent to a condenser-reboiler where it partially vaporizes the bottom liquid to form a vaporized gas

Methodology Applied
Scientific EffectPartial vaporization: Evaporation

Data Source

PatentEP2673582B1Process and device for the cryogenic separation of a methane-rich stream
Publication Date: 2018.10.10 LAIR LIQUIDE SA POUR LETUDE & LEXPLOITATION DES PROCEDES GEORGES CLAUDE
  • EP2673582B1 patent drawingFigure 1
  • EP2673582B1 patent drawingFigure 2

AI summary

In a process for the cryogenic separation of a methane-rich feed stream containing between 3 and 35% of oxygen and also nitrogen, the feed stream is cooled in order to produce a cooled stream, at least one portion of the cooled stream is sent to a distillation column (6), a bottom stream is withdrawn from the distillation column, the bottom stream being enriched in methane compared to the feed stream, a stream enriched in oxygen compared to the feed stream is withdrawn from the distillation column, and a nitrogen-rich stream (20, 21) is sent to the column.