Crystallisation-Assisted Membrane Distillation for Desalination

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Solution Overview

Problem

Current membrane distillation processes for desalination face issues such as crystallization on membrane surfaces leading to clogging, high energy consumption, and contamination risks due to the use of foreign substances, particularly when dealing with high salt concentrations like seawater or brine.

Innovation Solution

A process that prevents or reduces crystallization on membrane surfaces by using a crystallization agent with higher water solubility than the target compound, typically an inorganic salt, to induce crystallization of the first compound, followed by membrane separation to produce pure water, where the crystallization agent is recycled and minimizes contamination risks.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If membrane distillation is used for desalination of high salt concentration streams, then separation of pure water is achieved, but crystallization occurs on membrane surfaces causing clogging and flux decrease

Engineering Contradiction:
Improvemembrane performance stabilityVSAvoidcrystallization on membrane surface
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent applies preliminary action by adding a crystallization agent to the feed stream before membrane distillation to induce crystallization of salts in the bulk solution. This prevents supersaturation at the membrane surface, thereby avoiding crystallization on the membrane and subsequent clogging, while maintaining stable membrane performance throughout the process

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent introduces a crystallization agent as an intermediary substance that mediates between the high salt concentration feed stream and the membrane distillation process. This agent induces crystallization in the bulk solution, acting as a buffer to prevent direct crystallization on the membrane surface, thus protecting the membrane from clogging

Inventive Principle:
Principle #24Intermediary (Mediator)

2Reliability

If thermal evaporation methods are used for desalination, then pure water and concentrated brine are produced, but high energy consumption and scaling problems occur

Engineering Contradiction:
Improvedesalination effectivenessVSAvoidenergy consumption
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

The patent applies parameter changes by modifying the thermal process parameters - using lower temperatures combined with crystallization agent addition. This shifts the separation mechanism from pure thermal evaporation to a combined crystallization-membrane separation process, reducing energy consumption while maintaining desalination effectiveness and avoiding scaling

Inventive Principle:
Principle #35Parameter changes

3Reliability

If antisolvent induced crystallisation is used to prevent membrane clogging, then crystallization is induced, but foreign substances are introduced causing product contamination

Engineering Contradiction:
Improvemembrane performance stabilityVSAvoidproduct contamination
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent applies parameter changes by selecting a crystallization agent with specific properties - high water solubility and common ion effect - rather than using traditional antisolvents. This changes the crystallization mechanism from antisolvent-induced to supersaturation-controlled, preventing foreign substance contamination while maintaining membrane performance stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies homogeneity by using a crystallization agent that is chemically compatible with the feed stream (same ion type, high water solubility). This ensures the agent mixes uniformly with the feed without introducing foreign substances, maintaining product purity while preventing membrane clogging through controlled crystallization

Inventive Principle:
Principle #33Homogeneity

4Reliability

If reverse osmosis is used for desalination, then separation is achieved, but high pressures are required especially at high osmotic pressure

Engineering Contradiction:
Improveseparation qualityVSAvoidoperating pressure
Core Design Contradiction:
ReliabilityVSStress or pressure

Solution Approach 1:

The patent applies parameter changes by shifting from pressure-driven reverse osmosis to temperature-driven membrane distillation combined with crystallization. This changes the driving force parameter from high pressure to moderate temperature difference, reducing mechanical stress while maintaining separation quality through the combined crystallization-membrane separation mechanism

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively separates the target compound from the feed stream, reducing energy costs and contamination risks, while maintaining membrane integrity and efficiency by recycling the crystallization agent and producing a high-purity water product.

Implementation Method 1

adding a crystallisation agent to the feed stream, thereby causing crystallisation of at least part of the first compound from the feed stream

Methodology Applied
Scientific EffectCrystallisation: Crystallisation

Implementation Method 2

the crystallisation agent has a higher water solubility than the first compound

Methodology Applied
Scientific EffectSolubility reduction: Precipitation

Implementation Method 3

the liquid stream is subjected to a membrane separation process, comprising membrane distillation or osmotic distillation

Methodology Applied
Scientific EffectMembrane distillation: Distillation

Implementation Method 4

membrane distillation (MD), osmotic distillation (OD)

Methodology Applied
Scientific EffectVapor pressure difference: Vapour Pressure

Data Source

PatentEP2855355B1Crystallisation assisted membrane separation process
Publication Date: 2021.03.31 STICHTING WAGENINGEN RES
  • EP2855355B1 patent drawingFigure 1~2

AI summary

The invention is directed to a process for separating a compound from an aqueous feed stream wherein said compound is dissolved. The process of the invention comprises - adding a crystallisation agent to said feed stream, thereby causing at least part of said first compound to crystallise, resulting in a mixture of crystals and a liquid, - separating at least part of the crystals from the liquid, leaving a supernatant, - subjecting at least part of the supernatant to a membrane separation process, producing a concentrate; wherein the crystallisation agent comprises a second compound with a higher solubility in water than the first compound; wherein said membrane separation process comprises membrane distillation, osmotic distillation or a combination of both.