Cu Nanoparticle Ink Dispersion Without Dispersants

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing inkjet printing processes face challenges with dispersing Cu and CuO nanoparticles due to aggregation, clogging of nozzles, and substrate limitations, particularly requiring dispersants that increase energy demands and lead to volumetric shrinkage issues.

Innovation Solution

A process for preparing an ink with Cu and CuO nanoparticles that achieves dispersibility and stability without additives, by controlling oxygen states, using RF plasma treatment, vacuum drying, and quantifying ionic impurities, with specific conditions for zeta-potential, particle size, and interparticle distance, and using a polar solvent with low vapor pressure.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If dispersants are used to disperse Cu and CuO nanoparticles, then dispersibility is improved, but energy consumption increases and volumetric shrinkage occurs

Engineering Contradiction:
ImprovedispersibilityVSAvoidenergy consumption
Core Design Contradiction:
Stability of the object's compositionVSUse of energy by moving object

Solution Approach 1:

The invention extracts and removes dispersants from the ink composition entirely. By controlling the oxygen state of Cu and CuO nanoparticles (maintaining specific ratios of metallic Cu, Cu2O, and CuO), the particles achieve stable dispersion without requiring any dispersant additives, thereby eliminating the energy consumption and volumetric shrinkage issues associated with dispersant removal

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the chemical composition parameters of the nanoparticle mixture by precisely controlling the ratios of metallic Cu, Cu2O, and CuO. This parameter change in the oxygen state of the particles provides inherent dispersibility without needing external dispersants, resolving the contradiction between dispersibility and energy consumption

Inventive Principle:
Principle #35Parameter changes

2Stability of the object's composition

If dispersants are used to disperse Cu and CuO nanoparticles, then dispersibility is improved, but volumetric shrinkage and cracking occur

Engineering Contradiction:
ImprovedispersibilityVSAvoidvolumetric shrinkage
Core Design Contradiction:
Stability of the object's compositionVSObject-generated harmful factors

Solution Approach 1:

The invention extracts and removes dispersants from the ink composition entirely. By controlling the oxygen state of Cu and CuO nanoparticles (maintaining specific ratios of metallic Cu, Cu2O, and CuO), the particles achieve stable dispersion without requiring any dispersant additives, thereby eliminating the volumetric shrinkage and cracking issues that occur when dispersants are removed after deposition

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The nanoparticle mixture serves its own dispersion function through its controlled oxygen state composition. The specific ratio of metallic Cu, Cu2O, and CuO provides inherent steric and electrostatic repulsion that maintains particle separation without external dispersants, preventing the harmful volumetric shrinkage that would otherwise occur

Inventive Principle:
Principle #25Self-service

3Reliability

If high heating temperature is used for conductorization, then conductivity is improved, but substrate damage occurs

Engineering Contradiction:
ImproveconductivityVSAvoidsubstrate damage
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The invention changes the chemical composition parameters of the nanoparticle mixture by precisely controlling the ratios of metallic Cu, Cu2O, and CuO. This parameter change enables effective conductorization at lower temperatures because the mixed oxidation states facilitate sintering and conductivity formation without requiring the high temperatures (200°C or higher) that would damage heat-sensitive substrates

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite nanoparticle material consisting of metallic Cu, Cu2O, and CuO in specific ratios. This composite structure provides both the reducibility needed for low-temperature conductorization and the final conductivity required for functional wiring, eliminating the need for high-temperature processing that would damage the substrate

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The ink exhibits excellent dispersibility and stability, allowing for precise wiring patterns without nozzle clogging and enabling use on substrates with low heat resistance, while reducing energy requirements and preventing volumetric shrinkage.

Implementation Method 1

using RF plasma treatment

Methodology Applied
Scientific EffectPlasma treatment: Plasma

Implementation Method 2

vacuum drying

Methodology Applied
Scientific EffectVacuum drying: Vacuum

Data Source

PatentEP2479227B1Process for making printing ink
Publication Date: 2015.01.07 RESONAC CORP
  • EP2479227B1 patent drawingFigure 1~2
  • EP2479227B1 patent drawingFigure 3~5
  • EP2479227B1 patent drawing

AI summary

Disclosed is a printing ink comprising Cu- and/or CuO-containing metal nanoparticles, which obtains excellent dispersion properties and successive dispersion stability without using additives such as dispersing agents. Specifically disclosed is a printing ink that comprises Cu- and/or CuO-containing metal nanoparticles and has no more than 2,600 ppm of ionic impurities in the total solid content. The printing ink is obtained by dispersing the Cu- and/or CuO-containing metal nanoparticles, which have no more than 2,600 ppm of ionic impurities in the total solid content, in a dispersion medium.