Curable Electronics Composition for Chip Package Stress Relief

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Solution Overview

Problem

Conventional underfill materials for chip packages face challenges in providing low coefficient of thermal expansion (CTE), high thermal conductivity, moderate modulus, and tunable glass transition temperature, while also being easy to use and apply, especially in next-generation electronic applications where stress reduction and improved reliability are critical.

Innovation Solution

A curable electronics composition comprising a matrix material with a filler, derived from methylene malonate, multifunctional methylene, or methylene beta ketoester monomers, which can be tailored to achieve a CTE of less than 30 ppm/°C, cure at ambient temperature, and exhibit low viscosity, providing adhesion and strain relief in chip packages.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional polymer composites or epoxy resins are used as underfill materials, then the underfill can buffer thermal stresses, but the CTE matching with interconnects is poor and stress reduction is insufficient

Engineering Contradiction:
Improvestress reduction in interconnectsVSAvoidCTE matching with interconnects
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent changes the chemical composition parameters of the underfill material by using cyanate ester or phenolic resin matrices with specific inorganic filler loadings (5-95 wt%) to achieve CTE values between 3-15 ppm/°C, which closely matches the CTE of solder interconnects (5-20 ppm/°C), thereby reducing thermal stress

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates composite underfill materials by combining organic resin matrices (cyanate ester or phenolic resin) with inorganic fillers (silica, alumina, titania, zirconia, or boron nitride) in specific ratios, where the inorganic fillers dominate the CTE behavior to achieve better matching with interconnects while maintaining structural integrity

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If high inorganic filler loading is used to reduce CTE, then CTE matching improves, but the viscosity of the uncured composition increases and flow properties deteriorate

Engineering Contradiction:
ImproveCTE of underfill materialVSAvoidflow properties prior to cure
Core Design Contradiction:
Stability of the object's compositionVSEase of operation

Solution Approach 1:

The patent optimizes the viscosity parameter by selecting resin matrices (cyanate ester or phenolic resin) with inherently lower viscosity and by controlling the particle size distribution and surface treatment of inorganic fillers, enabling high filler loadings (5-95 wt%) while maintaining pourable flow properties and complete gap filling capability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent utilizes the porous or surface-modified structure of inorganic fillers to improve dispersion and reduce agglomeration, allowing high filler content without excessive viscosity increase, while the resin matrix penetrates and binds the filler particles effectively

Inventive Principle:
Principle #31Porous materials

3Reliability

If the underfill material requires high temperature curing, then complete curing and adhesion are achieved, but thermal stress during curing increases and processing complexity increases

Engineering Contradiction:
Improveadhesion and curing completenessVSAvoidcuring temperature
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The patent changes the curing temperature parameter from conventional high temperatures to ambient or room temperature curing by selecting cyanate ester or phenolic resin matrices that undergo spontaneous or catalyzed curing at low temperatures, reducing thermal stress during processing while achieving complete curing and strong adhesion

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent enables self-service curing where the underfill material cures automatically at ambient temperature through the chemical properties of cyanate ester or phenolic resin, eliminating the need for external heating equipment and complex curing cycles, thereby simplifying processing while ensuring complete adhesion

Inventive Principle:
Principle #25Self-service

4Strength

If the glass transition temperature of the underfill is too low, then the material remains flexible and absorbs stress, but the material may soften at operating temperatures; if too high, then the material maintains structural integrity but becomes brittle and less effective at stress buffering

Engineering Contradiction:
Improvestructural integrity of underfillVSAvoidbrittleness at high Tg
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The patent optimizes the glass transition temperature parameter by selecting cyanate ester or phenolic resin matrices with inherent Tg values that provide the desired balance, and by adjusting the inorganic filler content and type to modify the polymer-filler interface interactions, achieving a Tg that ensures both structural integrity and stress buffering capability at operating temperatures

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively reduces thermal mechanical stress in chip packages, allows for room temperature curing, and offers improved reliability by matching the CTE of chip and substrate materials, while being easy to apply and use, thus enhancing the performance of chip packaging and electronics materials.

Implementation Method 1

The mixture can have a cure temperature of around ambient or room temperature

Methodology Applied
Scientific EffectAmbient temperature curing:

Implementation Method 2

They can include inorganic particles in a polymer matrix such as silica (SiO2) to modify the coefficient of thermal expansion (CTE) of the underfill. This allows for more closely matching the CTE of the underfill to the material used to form the electrical interconnects

Methodology Applied
Scientific EffectCoefficient of thermal expansion matching: Thermal Expansion

Implementation Method 3

Such underfill compositions are known for example from JP2004304125 and WO2006/098514. Integrated circuits and their interconnects generate heat. This heat induces thermal expansion in the chip, interconnects, and external circuitry. Since these structures are typically formed from different materials with different coefficients of thermal expansion, stresses can develop between the chip and external circuitry

Methodology Applied
Scientific EffectStress buffering:

Data Source

PatentEP2926368B1Electronic assembly
Publication Date: 2020.04.08 SIRRUS
  • EP2926368B1 patent drawingFigure 1~2
  • EP2926368B1 patent drawingFigure 3
  • EP2926368B1 patent drawingFigure 4

AI summary

An electronics composition includes a curable matrix material and, optionally, a filler material disposed within the matrix material. The cured matrix material includes an oligomer or polymer material derived from a compound selected from a methylene malonate monomer, a multifunctional methylene monomer, a methylene beta ketoester monomer, a methylene beta diketone monomer, or a mixture thereof.