Containers comprising polyester compositions which comprise cyclobutanediol

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Solution Overview

Problem

Current plastic materials for containers, such as PET and polycarbonate, face challenges with high-heat applications, poor barrier properties, and difficulties in processing due to rapid crystallization and high melt viscosity, which limits their use in high-temperature conditions and affects their mechanical properties like impact strength and chemical resistance.

Innovation Solution

A polyester composition comprising terephthalic acid, 2,2,4,4-tetramethyl-1,3-cyclobutanediol, and 1,4-cyclohexanedimethanol with specific mole percentages, offering a balance of high impact strength, heat resistance, chemical resistance, and processability, while maintaining low ductile-to-brittle transition temperatures and low densities, allowing for the formation of amorphous or semicrystalline articles.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If PET is used for container production, then good barrier properties are achieved, but high-heat application performance deteriorates

Engineering Contradiction:
Improvebarrier propertiesVSAvoidhigh-heat application performance
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The patent uses a copolyester composition combining PCT (poly(1,4-cyclohexylenedimethylene) terephthalate) with other polyester components to create a composite material that maintains good barrier properties while achieving high-heat resistance, allowing containers to withstand pasteurization and retort applications

Inventive Principle:
Principle #40Composite materials

2Temperature

If polycarbonate is used for high-heat containers, then heat resistance is improved, but barrier properties deteriorate

Engineering Contradiction:
Improveheat resistanceVSAvoidbarrier properties
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

The patent develops a copolyester composition that combines the heat resistance of polycarbonate-like structures with the barrier properties of polyester, creating a composite material that achieves both high-heat tolerance and good barrier performance simultaneously

Inventive Principle:
Principle #40Composite materials

3Temperature

If PCT is used for container production, then high-heat resistance is achieved, but crystallization rate becomes too rapid for processing

Engineering Contradiction:
Improveheat resistanceVSAvoidcrystallization rate
Core Design Contradiction:
TemperatureVSEase of manufacture

Solution Approach 1:

The patent modifies the crystallization rate of PCT by changing compositional parameters - specifically by incorporating copolymer components that slow down crystallization, allowing sufficient time for container formation processes while maintaining the desired heat resistance properties

Inventive Principle:
Principle #35Parameter changes

4Loss of time

If ethylene glycol is added to PCT to slow crystallization, then crystallization half-time is improved, but glass transition temperature and impact strength deteriorate

Engineering Contradiction:
Improvecrystallization half-timeVSAvoidimpact strength
Core Design Contradiction:
Loss of timeVSStrength

Solution Approach 1:

The patent optimizes the compositional parameters by selecting specific copolymer components and ratios that slow crystallization without significantly compromising glass transition temperature and impact strength, unlike ethylene glycol modification

Inventive Principle:
Principle #35Parameter changes

5Temperature

If bisphenol A polycarbonate is used for high-performance containers, then heat resistance and impact strength are improved, but melt viscosity becomes too high for processing

Engineering Contradiction:
Improveheat resistanceVSAvoidmelt processability
Core Design Contradiction:
TemperatureVSEase of manufacture

Solution Approach 1:

The patent creates a copolyester composition that achieves heat resistance similar to bisphenol A polycarbonate but with significantly improved melt processability, eliminating the high viscosity problem while maintaining high-temperature performance

Inventive Principle:
Principle #40Composite materials

6Strength

If polymers with high inherent viscosity are used, then mechanical strength is improved, but processability on standard equipment deteriorates

Engineering Contradiction:
Improvemechanical strengthVSAvoidprocessability
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The patent optimizes the inherent viscosity parameter to a specific range that provides adequate mechanical strength while ensuring compatibility with standard industrial processing equipment, balancing material performance with manufacturability

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentEP2329856B1Containers comprising polyester compositions which comprise cyclobutanediol
Publication Date: 2019.07.24 EASTMAN CHEM CO
  • EP2329856B1 patent drawingFigure 1
  • EP2329856B1 patent drawingFigure 2
  • EP2329856B1 patent drawingFigure 3

AI summary

Described are bottle(s) comprising polyesters comprising (a) a dicarboxylicacidcomponent comprising terephthalic acids residues; optionally, aromatic dicarboxylic acid or aliphatic dicarboxylic acid residues; 2,2,4,4-tetramethyl-1,3-cyclobutanediol residues; and 1,4-cyclohexanedimethanol residues.