Cynaropicrin Extraction Using Ultrasonic Cavitation

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Solution Overview

Problem

Current methods for extracting cynaropicrin from Cynara cardunculus leaves result in lower concentrations and longer extraction times, often requiring additional purification steps and environmentally aggressive solvents, whereas there is a need for higher yields and reduced environmental impact.

Innovation Solution

The use of solid-liquid batch extraction, ultrasonic, microwave, and pressurized liquid extraction methods with solvents like ethanol, ethyl acetate, and ethanol/water mixtures, which reduce extraction time and increase cynaropicrin concentration without the need for additional purification steps, using environmentally friendly solvents and lower temperatures.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional solid-liquid batch extraction is used, then extraction simplicity is maintained, but extraction time is long (7 hours) and cynaropicrin concentration is low (55 mg/g dry weight)

Engineering Contradiction:
Improvecynaropicrin concentrationVSAvoidextraction time
Core Design Contradiction:
ProductivityVSLoss of time

Solution Approach 1:

The patent replaces conventional mechanical batch extraction with ultrasonic extraction technology. The ultrasonic waves create cavitation bubbles that collapse and generate localized high energy, dramatically enhancing the extraction efficiency of cynaropicrin from Cynara cardunculus leaves. This substitution reduces extraction time from 7 hours to significantly shorter durations while increasing cynaropicrin concentration yield.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent optimizes extraction parameters including using ethanol/water mixtures at specific ratios (e.g., 70:30, 80:20), controlling extraction temperature (40-60°C), and adjusting solid-liquid ratios. These parameter changes enable higher cynaropicrin extraction efficiency compared to conventional methods, achieving concentrations up to 40 mg/g dry weight with reduced extraction time.

Inventive Principle:
Principle #35Parameter changes

2Object-affected harmful factors

If conventional extraction methods are used, then extraction process is simple, but environmentally aggressive solvents are required

Engineering Contradiction:
Improveenvironmental impactVSAvoidcynaropicrin concentration
Core Design Contradiction:
Object-affected harmful factorsVSProductivity

Solution Approach 1:

The patent changes the solvent system from aggressive conventional solvents to environmentally friendly ethanol/water mixtures. By optimizing the ethanol concentration (e.g., 70%, 80% v/v) and extraction parameters, the method achieves high cynaropicrin extraction efficiency (up to 40 mg/g dry weight) while eliminating the need for toxic solvents, thus reducing environmental impact and harmful factors.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If additional purification steps are added, then cynaropicrin purity is improved, but process complexity and cost increase

Engineering Contradiction:
Improvecynaropicrin purityVSAvoidprocess steps
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent replaces complex multi-step purification processes with a single ultrasonic extraction step using optimized ethanol/water mixtures. The ultrasonic cavitation effect selectively extracts cynaropicrin with high efficiency, producing extracts with sufficient purity (up to 40 mg/g dry weight) that eliminate the need for additional chromatography or fractionation steps, thereby simplifying the overall process while maintaining manufacturing precision.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

These methods achieve higher cynaropicrin concentrations (up to 27-40 mg/g dry weight) with reduced extraction times and lower energy costs, while avoiding the use of aggressive solvents, thus enhancing the efficiency and sustainability of the extraction process.

Implementation Method 1

extraction of the lyophilised biomass with the solvent selected in the previous step in a closed container protected from light, subjected to the action of bath ultrasound equipment or with a probe

Methodology Applied
Scientific EffectUltrasonic cavitation: Cavitation

Implementation Method 2

The container is subjected to the action of bath ultrasound equipment or with a probe during the extraction step

Methodology Applied
Scientific EffectUltrasonic vibration: Ultrasonic Vibration

Implementation Method 3

The container is subjected to the action of microwave equipment during the extraction step

Methodology Applied
Scientific EffectMicrowave heating: Microwave Radiation

Implementation Method 4

extraction by pressurized liquid

Methodology Applied
Scientific EffectPressurized liquid extraction: Pressurisation

Data Source

PatentEP3466936B1Extraction processes for cynaropicrin present in the leaves of cynara cardunculus l.
Publication Date: 2020.06.24 CEBAL CENT DE BIOTECHA AGRI E AGRO ALIMENTAR DO ALENTEJO

AI summary

The present invention relates to methods for the extraction of the sesquiterpene lactone cynaropicrin, present in leaves of Cynara cardunculus. The invention contemplates the extraction of cynaropicrin, present in thistle leaves (Cynara cardunculus), where, before the extractive process, the biomass undergoes a size reduction in order to obtain a grain size of less than 400 µm. After this first step, the biological material in the present invention undergoes several types of independent extraction: solid-liquid batch, ultrasounds, microwaves or pressurized liquid solvent extraction. In the present invention, pure solvents, such as ethanol, ethyl acetate, as well as solvent mixtures, such as ethanol/water, are also presented as extraction solvents. The extraction process is controlled in relation to time, temperature, solid-liquid ratio and solvent variables for the set of processes shown, and depending on the extraction process, controlled in relation to stirring, ultrasonic power, microwave power and number of cycles of extraction. These processes of cynaropicrin extraction have potential for application in the nutraceutical, pharmaceutical and chemical industries.