CZTS Photovoltaic Coating via Low-Temperature Sintering

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Solution Overview

Problem

Current photovoltaic device manufacturing processes, particularly for Copper Zinc Tin Selenium/Sulfide (CZTS) devices, rely on hazardous materials and high-temperature/vacuum processes, leading to high costs and inefficiencies, necessitating the development of safer, lower-temperature, and more cost-effective methods.

Innovation Solution

A method involving the use of a coating liquid containing semiconducting particles and additives, where the solvent is evaporated and the mixture is sintered at a lower temperature (400-500°C) to form a semiconductor light absorption layer, using additives that stabilize the particles and facilitate dense packing, reducing the need for hazardous materials and high-temperature processes.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If high-temperature and vacuum-based processes are used to manufacture CZTS PV devices, then power conversion efficiency is improved, but manufacturing cost increases and process complexity increases

Engineering Contradiction:
Improvepower conversion efficiencyVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent changes the temperature parameter from high-temperature vacuum processes to low-temperature atmospheric processes (below 400°C). The coating method transitions from vacuum deposition to liquid coating followed by low-temperature sintering, fundamentally altering the process parameters to reduce manufacturing cost while maintaining acceptable efficiency

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces the mechanical vacuum system with a liquid coating system. Instead of using vacuum-based deposition methods, the invention uses liquid precursors that are coated onto the substrate and then sintered at low temperatures, eliminating the need for expensive vacuum equipment

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Reliability

If hazardous materials are used in CZTS PV device manufacturing, then power conversion efficiency is improved, but safety hazards increase

Engineering Contradiction:
Improvepower conversion efficiencyVSAvoidsafety hazards
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent uses low-cost, non-hazardous liquid precursor materials that can be easily handled and disposed of. Instead of using toxic materials in solid or vapor form that require special handling, the invention employs stable liquid solutions that pose minimal safety risks

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent introduces liquid precursor compounds as intermediaries that contain the necessary metal elements (Cu, Zn, Sn, S, Se) in a safe, soluble form. These liquid intermediaries replace hazardous materials and can be applied using simple coating techniques without special safety precautions

Inventive Principle:
Principle #24Intermediary (Mediator)

3Manufacturing precision

If vacuum processes are used for manufacturing PV devices, then material deposition quality is improved, but process speed decreases

Engineering Contradiction:
Improvematerial deposition qualityVSAvoidprocess speed
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent replaces slow vacuum deposition processes with rapid liquid coating methods. The liquid precursor can be applied quickly using dip-coating, spin-coating, or spray-coating techniques, and the subsequent low-temperature sintering process is faster than vacuum-based material deposition

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent changes the deposition mechanism from vacuum-phase material transport to liquid-phase precursor application. This parameter change enables much faster processing speeds while the controlled sintering process ensures high-quality material formation

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the production of photovoltaic devices with improved power conversion efficiency while minimizing the use of dangerous materials and reducing manufacturing costs through a lower-temperature process, enhancing the throughput and safety of the production process.

Implementation Method 1

evaporating the solvent from the stack by applying heat

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 2

sintering the stack to form the SLAL

Methodology Applied
Scientific EffectSintering: Sintering

Data Source

PatentEP2786419B1Method of manufacturing a photovoltaic device
Publication Date: 2020.02.12 KONICA MINOLTA SYSTEMS LABORATORY INC
  • EP2786419B1 patent drawingFigure 1
  • EP2786419B1 patent drawingFigure 2
  • EP2786419B1 patent drawingFigure 3

AI summary

A photovoltaic device and a method of making a photovoltaic device that includes a stack of layers, including a substrate and an electrode layer. The photovoltaic device includes a semiconductor light absorption layer that is formed on the stack by a coating liquid that includes a plurality of semiconducting particles. The coating liquid may also include a solvent and a plurality of additive molecules. The photovoltaic device also includes a transparent conducting layer disposed on the semiconductor light absorption layer and a grid electrode disposed on the transparent conducting layer.